We present a scheme for correcting the spectral fluctuations of high-harmonic radiation. We show that the fluctuations of the extreme-ultraviolet (XUV) spectral power density can be predicted solely by monitoring the generating laser pulses; this method is in contrast with traditional balanced detection used in optical spectroscopy, where a replica of the signal is monitored. Such possibility emerges from a detailed investigation of high-harmonic generation (HHG) noise. We find that in a wide parameter range of the HHG process, the XUV fluctuations are dominated by a spectral blueshift, which is correlated to the near-infrared (NIR) driving laser intensity variation. Numerical simulations support our findings and suggest that non-adiabatic blueshift is the main source of XUV fluctuations. A straightforward post-processing of the XUV spectra allows for noise reduction and improved precision of attosecond transient absorption experiments. The technique is readily transferable to attosecond transient reflectivity and potentially to attosecond photoelectron spectroscopy.
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http://dx.doi.org/10.1364/OE.27.007886 | DOI Listing |
J Phys Chem A
January 2025
Department of Chemistry, University of Malaya, 50603 Kuala Lumpur, Malaysia.
This study investigates the motion of an electron in a Coulomb potential driven by an intense linearly polarized XUV laser pulse analyzed using Gordon-Volkov wave functions. The wave function is decomposed into spherical partial waves to model the scattered electron wave packet after the recollision with a proton. This interaction triggers high harmonic generation, producing coherent X-ray pulses with frequencies that are integer multiples of the XUV field.
View Article and Find Full Text PDFNature
January 2025
Department of Physics and Astronomy, University of California, Los Angeles, Los Angeles, CA, USA.
Microscopy and crystallography are two essential experimental methodologies for advancing modern science. They complement one another, with microscopy typically relying on lenses to image the local structures of samples, and crystallography using diffraction to determine the global atomic structure of crystals. Over the past two decades, computational microscopy, encompassing coherent diffractive imaging (CDI) and ptychography, has advanced rapidly, unifying microscopy and crystallography to overcome their limitations.
View Article and Find Full Text PDFJ Chem Theory Comput
January 2025
State Key Laboratory for Mesoscopic Physics and Collaborative Innovation Center of Quantum Matter, School of Physics, Peking University, Beijing 100871, China.
We report on continuous high-harmonic generation (HHG) at 1 kHz repetition rate from a liquid-sheet plasma mirror driven by relativistic-intensity near-single-cycle light transients. Through precise control of both the surface plasma density gradient and the driving light waveform, we can produce highly stable and reproducible extreme ultraviolet spectral quasi-continua, expected to correspond to the generation of stable kHz-trains of isolated attosecond pulses in the time domain. This confirms the exciting potential of liquid-sheet targets as one of the building blocks of future high-power attosecond lasers.
View Article and Find Full Text PDFJ Chem Theory Comput
January 2025
Max Planck Institute for the Structure and Dynamics of Matter, Luruper Ch 149, Hamburg 22761, Germany.
High-harmonic generation (HHG) is a nonlinear process in which a material sample is irradiated by intense laser pulses, causing the emission of high harmonics of incident light. HHG has historically been explained by theories employing a classical electromagnetic field, successfully capturing its spectral and temporal characteristics. However, recent research indicates that quantum-optical effects naturally exist or can be artificially induced in HHG, such as entanglement between emitted harmonics.
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