Photonic metasurfaces, a kind of 2D structured medium, represent a novel platform to manipulate the propagation of light at subwavelength scale. In linear optical regime, many interesting topics such as planar meta-lenses, metasurface optical holography, and so on have been widely investigated. Recently, metasurfaces have gone into the nonlinear optical regime. While it is recognized that the local symmetry of the meta-atoms plays a vital role in determining the polarization, phase, and intensity of the nonlinear waves, much less attention has been paid to the global symmetry of the nonlinear metasurfaces. According to the Penrose tiling and the newly proposed hexagonal quasicrystalline tiling, nonlinear optical quasicrystal metasurfaces are designed and fabricated based on the geometric-phase-controlled plasmonic meta-atoms with local rotational symmetry. It is found that the far-field radiation behavior of second harmonic generation waves are determined by both the tiling schemes of quasicrystal metasurfaces and the local symmetry of meta-atoms they consist of. The proposed concept may open new avenues for designing nonlinear optical sources with metasurface crystals.
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http://dx.doi.org/10.1002/adma.201901188 | DOI Listing |
Sci Adv
January 2025
Guangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications, Institute of Photonics Technology, Jinan University, Guangzhou 510632, China.
Artificial nanostructures with ultrafine and deep-subwavelength features have emerged as a paradigm-shifting platform to advanced light-field management, becoming key building blocks for high-performance integrated optoelectronics and flat optics. However, direct optical inspection of integrated chips remains a missing metrology gap that hinders quick feedback between design and fabrications. Here, we demonstrate that photothermal nonlinear scattering microscopy can be used for direct imaging and resolving of integrated optoelectronic chips beyond the diffraction limit.
View Article and Find Full Text PDFJ Vis
January 2025
Vision and Control of Action (VISCA) Group, Department of Cognition, Development and Psychology of Education, Institut de Neurociències, Universitat de Barcelona, Barcelona, Catalonia, Spain.
The characterization of how precisely we perceive visual speed has traditionally relied on psychophysical judgments in discrimination tasks. Such tasks are often considered laborious and susceptible to biases, particularly without the involvement of highly trained participants. Additionally, thresholds for motion-in-depth perception are frequently reported as higher compared to lateral motion, a discrepancy that contrasts with everyday visuomotor tasks.
View Article and Find Full Text PDFJ Phys Chem A
January 2025
Department of Chemistry, University of Michigan, Ann Arbor, Michigan 48109, United States.
Given their molecular properties and electronic structure, graphyne and graphdiyne are promising materials with numerous applications in different fields of material science. Dehydrobenzoannules (DBAs) are candidates that can serve as building blocks for synthesizing and designing new 2D carbon allotropes; however, only a few graphynes have been produced on a practical scale. Herein, we present our investigation of three DBAs, which serve as a model to understand the relationship between the structure and property, contributing to 2D carbon allotropes' rational design and synthetic effort.
View Article and Find Full Text PDFNanomaterials (Basel)
January 2025
College of Electronic and Optical Engineering and College of Flexible Electronics (Future Technology), Nanjing University of Posts and Telecommunications, Nanjing 210023, China.
Silver gallium sulfide (AgGaS) is a ternary ABX-type semiconductor featuring a direct bandgap and high chemical stability. Structurally resembling diamond, AgGaS has gained considerable attention as a highly promising material for nonlinear optical applications such as second harmonic generation and optical parametric oscillation. In attempts to expand the research scope, on the one hand, AgGaS-derived bulk materials with similar diamond-like configurations have been investigated for the enhancement of nonlinear optics performance, especially the improvement of laser-induced damage thresholds and/or nonlinear coefficients; on the other hand, nanoscale AgGaS and its derivatives have been synthesized with sizes as low as the exciton Bohr radius for the realization of potential applications in the fields of optoelectronics and lighting.
View Article and Find Full Text PDFNanomaterials (Basel)
January 2025
Key Laboratory of Organic Integrated Circuit, Tianjin Key Laboratory of Molecular Optoelectronic Sciences & Ministry of Education, Department of Chemistry, School of Science, Tianjin University, Tianjin 300072, China.
The exploitation of high-performance third-order nonlinear optical (NLO) materials that have a favorable optical limit (OL) threshold is essential due to a rise in the application of ultra-intense lasers. In this study, a Cu-based MOF (denoted as Cu-bpy) was synthesized, and its third-order NLO and OL properties were investigated using the Z-scan technique with the nanosecond laser pulse excitation set at 532 nm. The Cu-bpy exhibits a typical rate of reverse saturable absorption (RSA) with a third-order nonlinear absorption coefficient of 100 cm GW and a favorable OL threshold of 0.
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