We use inelastic neutron scattering to study energy and wave vector dependence of spin fluctuations in SrCo_{2}As_{2}, derived from SrFe_{2-x}Co_{x}As_{2} iron pnictide superconductors. Our data reveal the coexistence of antiferromagnetic (AF) and ferromagnetic (FM) spin fluctuations at wave vectors Q_{AF}=(1,0) and Q_{FM}=(0,0)/(2,0), respectively. By comparing neutron scattering results with those of dynamic mean field theory calculation and angle-resolved photoemission spectroscopy experiments, we conclude that both AF and FM spin fluctuations in SrCo_{2}As_{2} are closely associated with a flatband of the e_{g} orbitals near the Fermi level, different from the t_{2g} orbitals in superconducting SrFe_{2-x}Co_{x}As_{2}. Therefore, Co substitution in SrFe_{2-x}Co_{x}As_{2} induces a t_{2g} to e_{g} orbital switching, and is responsible for FM spin fluctuations detrimental to the singlet pairing superconductivity.
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http://dx.doi.org/10.1103/PhysRevLett.122.117204 | DOI Listing |
NPJ Quantum Mater
January 2025
NIST Center for Neutron Research, Gaithersburg, MD 20899 USA.
The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry and points and disperse along the crystallographic -axis. In applied magnetic fields to at least = 11 T along the , the magnetism is found to be field-independent in the ( 0) plane.
View Article and Find Full Text PDFNat Commun
January 2025
Institute of Solid State Physics, TU Wien, 1040, Vienna, Austria.
Waterfalls are anomalies in the angle-resolved photoemission spectrum where the energy-momentum dispersion is almost vertical, and the spectrum strongly smeared out. These anomalies are observed at relatively high energies, among others, in superconducting cuprates and nickelates. The prevalent understanding is that they originate from the coupling to some boson, with spin fluctuations and phonons being the usual suspects.
View Article and Find Full Text PDFChem Commun (Camb)
January 2025
College of Chemistry and Materials Engineering, Wenzhou University, Wenzhou 325035, China.
Layered transition metal oxide (NaTMO) cathodes are considered highly appropriate for the practical applications of sodium-ion batteries (SIBs) owing to their facile synthesis and high theoretical capacity. Generally, the phase evolution behaviors of NaTMO during solid-state reactions at high temperature closely related to their carbon footprint, prime cost, and the eventual electrochemical properties, while the thermal stability in various desodiated states associated with wide temperature fluctuations are extremely prominent to the electrochemical properties and safety of SIB devices. Therefore, in this review, the influences of sintering conditions such as pyrolysis temperature, soaking time, and cooling rates on the phase formation patterns of NaTMO are summarized.
View Article and Find Full Text PDFNature
January 2025
Max-Planck-Institut für Quantenoptik, Garching, Germany.
Phys Rev Lett
December 2024
Université Grenoble Alpes, Grenoble INP, CEA, IRIG, PHELIQS, 38000 Grenoble, France.
The antiferromagnetic structure of Yb_{3}Ga_{5}O_{12} is identified by neutron diffraction experiments below the previously known transition at T_{λ}=54 mK. The magnetic propagation vector is found to be k=(1/2,1/2,0), an unusual wave vector in the garnet structure. The associated complex magnetic structure highlights the role of exchange interactions in a nearly isotropic system dominated by dipolar interactions and finds echoes with exotic structures theoretically proposed.
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