The half-life of Fe has been measured accurately by following the decay curve of three sources with a large pressurised proportional counter. An argon(90%)-methane(10%) mixture was used as counter gas, at atmospheric pressure (∼1 × 10 Pa) and at enhanced pressures of 5 × 10 Pa and 8 × 10 Pa (for 1 source), respectively. The first measurements were performed in 2001, but the experiment was executed more systematically between 2005 and 2018, covering a period of about 5 half-lives. The residuals from an exponential decay curve were of the order of 0.1% to 0.2% at 1 × 10 Pa, and 0.03% at 5 × 10 Pa and 8 × 10 Pa. The gain of stability with increased gas pressure was due to asymptotically reaching the maximum counting efficiency, resulting in lower sensitivity to pressure variations. The deduced half-life value of T(Fe) = 1006.70 (15) d or 2.7563 (4) a is more accurate than other data in literature, which are mutually discrepant. It is consistent with previous measurements at JRC with an X-ray defined solid angle counter.
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http://dx.doi.org/10.1016/j.apradiso.2019.01.008 | DOI Listing |
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