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Ionic Liquid-Functionalized Defective MOFs for Membrane-Based CO Separation: A Dual Optimization Approach for Interface and Transport.
ACS Appl Mater Interfaces
January 2025
School of Chemical Engineering, Zhengzhou University, Zhengzhou 450001, P. R. China.
Defective MOFs have been identified as promising candidates for efficient membrane-based separation applications. However, the utilization of defective MOFs in membrane gas separation is still in its infancy due primarily to the inefficient molecular differentiation induced by structural defects. Herein, we report a strategic combination of ionic liquid (IL) and defective UiO-66-NH MOF to ameliorate the CO/N selectivity within the highly permeable PIM-1 polymer.
View Article and Find Full Text PDFConstruction of predictive model for the risk of acute lactic acidosis in patients with ischemic stroke during the ICU stay: A study based on the medical information Mart for intensive care database.
J Clin Neurosci
January 2025
Department of Neurology, Beijing Shunyi Hospital, Beijing 101300, PR China. Electronic address:
Background: This study aims to identify the factors influencing the risk of lactic acidosis (LA) in patients with ischemic stroke (IS) and to develop a predictive model for assessing the risk of LA in IS patients during their stay in the intensive care unit (ICU).
Methods: A retrospective cohort design was employed, with data collected from the Medical Information Mart for Intensive Care (MIMIC)-III and MIMIC-IV databases spanning from 2001 to 2019. LA was defined as pH < 7.
Synthesis of α,β-Unsaturated Carbonyl Compounds via Cu/TEMPO/O2 Aerobic Catalytic System.
Chemistry
January 2025
Shihezi University, School of Chemistry and Chemical Engineering/State Key Laboratory Incubation Base for Green Processing of Chemical Engineering, North 4th Road, 832003, Shihezi, CHINA.
An N,N,N-type Cu(Ⅱ) complex-catalyzed desaturation method for converting alcohols, ketones, lactones, and lactams to their α,β-unsaturated carbonyl compounds is reported. The dehydrogenation reaction can be conducted with a green terminal oxidant O2 without requiring strong acid/base or stoichiometric oxidants. The Cu(Ⅱ) complex/TEMPO/O2 system uses a non-noble catalyst, and a green terminal oxidant as well as demonstrates high activity and functional group tolerance.
View Article and Find Full Text PDFLife-threatening dapagliflozin-associated euglycaemic diabetic ketoacidosis in a postoperative patient.
BMJ Case Rep
January 2025
Kasturba Medical College Mangalore, Mangalore, Karnataka, India
Euglyceamic diabetic ketoacidosis (EuDKA) is an uncommon but serious diabetes mellitus complication associated with risk factors such as fasting, surgery, pregnancy and, more recently, the use of sodium-glucose cotransporter-2 inhibitors (SGLT2i). This case is of a woman with type 2 diabetes and hypertension in her 50s who underwent an incarcerated umbilical hernia repair and abdominoplasty. Two days after discharge, she was readmitted with nausea, vomiting, loss of appetite, low-grade fever and breathing difficulty.
View Article and Find Full Text PDFThe adsorption behavior and mechanism of Cu(Ⅱ), Fe(Ⅱ) and Co(Ⅱ) on straw biochar and their Fenton-like performance for ciprofloxacin decontamination.
J Environ Manage
January 2025
Shaanxi Geology and Mining Hanzhong Geological Brigade Co., Ltd., Hanzhong, 723000, China.
In this study, the adsorption of aqueous Cu(Ⅱ), Fe(Ⅱ), and Co(Ⅱ) on biochars at diverse synthesized temperatures was evaluated. The optimal sample BC-800 achieved superior adsorption performance of Cu(Ⅱ), Fe(Ⅱ), and Co(Ⅱ) at 10-50 mg L initial concentration. Due to the larger surface area (349.
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