We investigate the ion gel gating of wide bandgap oxide, La-doped SrSnO films grown using radical-based molecular beam epitaxy. An applied positive bias resulted in a reversible electrostatic control of sheet resistance over 3 orders of magnitude at low temperature driving sample from Mott variable range hopping to a weakly localized transport. Analysis of low temperature transport behavior revealed electron-electron interaction and weak localization effects to be the dominant scattering mechanisms. A large voltage window (-4 V ≤ V ≤ +4 V) was obtained for reversible electrostatic doping of SrSnO films showing robustness of stannate with regards to redox chemistry with electrolyte gating irrespective of the bias type.
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http://dx.doi.org/10.1021/acsami.8b22034 | DOI Listing |
Sci Adv
November 2024
Department of Chemical Engineering and Materials Science, University of Minnesota-Twin Cities, Minneapolis, MN 55455, USA.
Nanoscale
June 2023
School of Microelectronics, Fudan University, Shanghai 200433, China.
ACS Appl Electron Mater
July 2022
Institute of Applied Physics, Department of Physics and Astronomy, Seoul National University, Seoul 08826, Republic of Korea.
Perovskite stannate SrSnO (SSO) is attracting attention as ultraviolet transparent conducting oxides (UV TCOs) due to its ultrawide band gap and high conductivity. Here, we investigate in detail the thickness-dependent electrical, structural, and optical properties of sequentially strain-relaxed La-doped SrSnO (SLSO) epitaxial thin films. We find that the SLSO films grow as an orthorhombic phase with in the direction under the tensile strain.
View Article and Find Full Text PDFRSC Adv
November 2021
Group of STCE-Energy Research Centre (ERC), Faculty of Science, Mohammed V University B. P. 1014 Rabat Morocco +212604710051.
The inorganic stannous-based perovskite oxide SrSnO has been utilized in various optoelectronic applications. Facilitating the synthesis process and engineering its properties, however, are still considered challenging due to several aspects. This paper reports on a thorough investigation of the influence of rare-earth (praseodymium) doping on the microstructural and optoelectronic properties of pure and Pr-doped SrSnO perovskite oxide thin films synthesized by a two-step simple chemical solution deposition route.
View Article and Find Full Text PDFNano Lett
December 2021
Department of Chemical Engineering and Materials Science, University of Minnesota - Twin Cities, Minneapolis, Minnesota 55455, United States.
Hysteretic magnetoresistance (MR) is often used as a signature of ferromagnetism in conducting oxide films and heterostructures. Here, magnetotransport is investigated in a nonmagnetic La-doped SrSnO film. A 12 nm La:SrSnO/2 nm SrSnO/GdScO (110) film with insulating behavior exhibited a robust hysteresis loop in the MR at < 5 K accompanied by an anomaly at ∼±3 T at < 2.
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