Using the 90-105 keV gamma-rays for determining Pu isotopic composition is studied for dilute Pu solutions (0.0001-0.05 μg/mm) as well as Pu-U mixed solutions. It is shown that for concentrations higher than 0.001 μg/mm Pu, results match well with those of mass spectrometric results. However, in mixed solutions, beyond 0.005 mg/mm U concentration, the errors on isotopic compositions of Pu increased as U content increased.

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http://dx.doi.org/10.1016/j.apradiso.2018.12.030DOI Listing

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