The first 2^{+} and 3^{-} states of the doubly magic nucleus ^{132}Sn are populated via safe Coulomb excitation employing the recently commissioned HIE-ISOLDE accelerator at CERN in conjunction with the highly efficient MINIBALL array. The ^{132}Sn ions are accelerated to an energy of 5.49 MeV/nucleon and impinged on a ^{206}Pb target. Deexciting γ rays from the low-lying excited states of the target and the projectile are recorded in coincidence with scattered particles. The reduced transition strengths are determined for the transitions 0_{g.s.}^{+}→2_{1}^{+}, 0_{g.s.}^{+}→3_{1}^{-}, and 2_{1}^{+}→3_{1}^{-} in ^{132}Sn. The results on these states provide crucial information on cross-shell configurations which are determined within large-scale shell-model and Monte Carlo shell-model calculations as well as from random-phase approximation and relativistic random-phase approximation. The locally enhanced B(E2;0_{g.s.}^{+}→2_{1}^{+}) strength is consistent with the microscopic description of the structure of the respective states within all theoretical approaches. The presented results of experiment and theory can be considered to be the first direct verification of the sphericity and double magicity of ^{132}Sn.
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http://dx.doi.org/10.1103/PhysRevLett.121.252501 | DOI Listing |
ACS Omega
September 2024
Laboratory for Chemical Computation and Modeling, Institute for Computational Science and Artificial Intelligence, Van Lang University, Ho Chi Minh 70000, Vietnam.
Density functional theory (DFT) calculations are carried out to determine the geometries and electronic and nonlinear optical (NLO) properties of the doubly doped gold clusters in three charge states M @ Au with M = W, Mo and = 0, ±1. At their lowest-lying equilibrium structures, the impurities that are vertically encapsulated inside a cylindrical gold framework, significantly enhance the stability and modify properties of the host. The presence of M units results in the formation of a tube-like ground state, which is identified for the first time for gold clusters.
View Article and Find Full Text PDFPhys Rev Lett
August 2024
Department of Physics, The University of Hong Kong, Pokfulam, Hong Kong, China.
Isomer spectroscopy of heavy neutron-rich nuclei beyond the N=126 closed shell has been performed for the first time at the Radioactive Isotope Beam Factory of the RIKEN Nishina Center. New millisecond isomers have been identified at low excitation energies, 985.3(19) keV in ^{213}Tl and 874(5) keV in ^{215}Tl.
View Article and Find Full Text PDFPhys Chem Chem Phys
August 2024
Molecule and Materials Modeling Laboratory and Department of Chemistry, Can Tho University, Can Tho, Vietnam.
The smallest triple ring tube-like gold clusters M@Au with M = Mo, W and = 1, 0, -1 are reported for the first time. Incorporation of an M dimer results in a remarkable modification of both atomic and electronic structures of the gold host. While the bare Au cluster exhibits a 3D cage shape, the doubly doped clusters M@Au in all charge states are found to prefer a tubular form composed of three five-membered Au rings in an anti-prism arrangement and stabilized by an M unit placed inside the tube-like Au gold framework.
View Article and Find Full Text PDFJ Phys Chem A
July 2024
College of Engineering, Huaqiao University, Quanzhou 362021, China.
Nat Nanotechnol
July 2024
Institute of Brain-Inspired Intelligence, National Laboratory of Solid State Microstructures, School of Physics, Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, China.
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