Probing the Combined Electromagnetic Local Density of Optical States with Quantum Emitters Supporting Strong Electric and Magnetic Transitions.

We experimentally demonstrate that the radiative decay rate of a quantum emitter is determined by the combined electric and magnetic local density of optical states (LDOS). A Drexhage-style experiment was performed for two distinct quantum emitters, divalent nickel ions in magnesium oxide and trivalent erbium ions in yttrium oxide, which both support nearly equal mixtures of isotropic electric dipole and magnetic dipole transitions. The disappearance of lifetime oscillations as a function of emitter-interface separation distance confirms that the electromagnetic LDOS refers to the total mode density, and thus similar to thermal emission, these unique electronic emitters effectively excite all polarizations and orientations of the electromagnetic field.