K-shell x-ray spectra of Li- to H-like ions have long been used to determine plasma conditions. The ratio of integrated line intensities is used to determine the temperature. At the density of non-local thermal dynamic equilibrium (NLTE) plasmas (n ≈ 10 cm), the K-shell spectrum is not very sensitive to density. We propose using the L-shell emission of open L-shell ions (C- to Li-like) as an alternative to determine both temperature and density of NLTE plasmas. First, the L-shell models of a mid-Z material need to be verified against the temperatures obtained using a K-shell spectrum of a low-Z material. A buried layer platform is being developed at the OMEGA laser to study the open L-shell spectra of NLTE plasmas of mid-Z materials. Studies have been done using a 250 m diameter dot composed of a layer of 1200 Å thick Zn between two 600 Å thick layers of Ti, in the center of a 1000 m diameter, 13 m thick beryllium tamper. Lasers heat the target from both sides for up to 3 ns. The size of the emitting volume vs time was measured with x-ray imaging (face-on and side-on) to determine the density. The temperature was measured from the Ti K-shell spectra. The use of this platform for the verification of atomic L-shell models is discussed.
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Appl Spectrosc
January 2025
Department of Physics & Applied Physics, Kennedy College of Sciences, University of Massachusetts Lowell, Lowell, Massachusetts, USA.
Under various atmospheric conditions, laser-induced breakdown spectroscopy (LIBS) is a powerful technique for elemental analysis, including in Earth- and Mars-like environments. However, understanding the plasma behavior and its dependence on ambient pressure and laser parameters remains a challenge. In this study, a numerical model based on a three-temperature Eulerian radiation framework under non-local thermodynamic equilibrium conditions is employed to investigate the interaction of a nanosecond laser pulse with a graphite target under helium (He) and carbon dioxide (CO atmospheres.
View Article and Find Full Text PDFPhys Rev E
February 2021
Center for Free-Electron Laser Science, DESY, Notkestrasse 85, 22607 Hamburg, Germany.
The advent of x-ray free-electron lasers (XFELs), which provide intense ultrashort x-ray pulses, has brought a new way of creating and analyzing hot and warm dense plasmas in the laboratory. Because of the ultrashort pulse duration, the XFEL-produced plasma will be out of equilibrium at the beginning, and even the electronic subsystem may not reach thermal equilibrium while interacting with a femtosecond timescale pulse. In the dense plasma, the ionization potential depression (IPD) induced by the plasma environment plays a crucial role for understanding and modeling microscopic dynamical processes.
View Article and Find Full Text PDFRev Sci Instrum
October 2018
Lawrence Livermore National Laboratory, 7000 East Ave., L-490, Livermore, California 94550, USA.
K-shell x-ray spectra of Li- to H-like ions have long been used to determine plasma conditions. The ratio of integrated line intensities is used to determine the temperature. At the density of non-local thermal dynamic equilibrium (NLTE) plasmas (n ≈ 10 cm), the K-shell spectrum is not very sensitive to density.
View Article and Find Full Text PDFPhys Plasmas
May 2017
Laboratory for Laser Energetics, Rochester, New York 14623, USA.
For several years, we have been calculating the radiation drive in laser-heated gold hohlraums using flux-limited heat transport with a limiter of 0.15, tabulated values of local thermodynamic equilibrium gold opacity, and an approximate model for not in a local thermodynamic equilibrium (NLTE) gold emissivity (DCA_2010). This model has been successful in predicting the radiation drive in vacuum hohlraums, but for gas-filled hohlraums used to drive capsule implosions, the model consistently predicts too much drive and capsule bang times earlier than measured.
View Article and Find Full Text PDFHigh Energy Density Phys
January 2017
National Institute of Standards and Technology, Gaithersburg, MD 20899-8422, USA.
We review the 9th NLTE code comparison workshop, which was held in the Jussieu campus, Paris, from November 30th to December 4th, 2015. This time, the workshop was mainly focused on a systematic investigation of iron NLTE steady-state kinetics and emissivity, over a broad range of temperature and density. Through these comparisons, topics such as modeling of the dielectronic processes, density effects or the effect of an external radiation field were addressed.
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