We show that it is possible to confine light in a volume of order 10 cubic wavelengths using only dielectric material. Low-index (air) cavities are simulated in high-index rod-connected diamond photonic crystals. These cavities show long storage times (Q-factors >10) even at the lowest volumes. Fabrication of such structures could open a new field of photon-level interactions.
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http://dx.doi.org/10.1364/OL.43.005202 | DOI Listing |
Science
May 2024
Faculty of Physics and CeNS, Ludwig-Maximilian-University Munich, München, 80539 Bayern, Germany.
Colloidal self-assembly allows rational design of structures on the micrometer and submicrometer scale. One architecture that can generate complete three-dimensional photonic bandgaps is the diamond cubic lattice, which has remained difficult to realize at length scales comparable with the wavelength of visible or ultraviolet light. In this work, we demonstrate three-dimensional photonic crystals self-assembled from DNA origami that act as precisely programmable patchy colloids.
View Article and Find Full Text PDFACS Nano
February 2021
School of Chemistry, University of Birmingham, Edgbaston, Birmingham B15 2TT, U.K.
Diamond-structured colloidal photonic crystals are much sought-after for their applications in visible light management because of their ability to support a complete photonic band gap (PBG). However, their realization self-assembly pathways is a long-standing challenge. This challenge is rooted in three fundamental problems: the design of building blocks that assemble into diamond-like structures, the sensitivity of the PBG to stacking faults, and ensuring that the PBG opens at an experimentally attainable refractive index.
View Article and Find Full Text PDFACS Appl Bio Mater
January 2020
Materials and Life Science Research Division, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea.
Self-assembled photonic crystals have proven to be a fascinating class of photonic materials for nonabsorbing structural colorizations over large areas and in diverse relevant applications, including tools for on-chip spectrometers and biosensors, platforms for reflective displays, and templates for energy devices. The most prevalent building blocks for the self-assembly of photonic crystals are spherical colloids and block copolymers (BCPs) because of the generic appeal of these materials, which can be crafted into large-area 3D lattices. However, because of the intrinsic limitations of these structures, these two building blocks are difficult to assemble into a direct rod-connected diamond lattice, which is considered to be a champion photonic crystal.
View Article and Find Full Text PDFWe show that it is possible to confine light in a volume of order 10 cubic wavelengths using only dielectric material. Low-index (air) cavities are simulated in high-index rod-connected diamond photonic crystals. These cavities show long storage times (Q-factors >10) even at the lowest volumes.
View Article and Find Full Text PDFWe propose a method to directly visualize the photonic band-structure of micrometer-sized photonic crystals using wide-angle spectroscopy. By extending Fourier imaging spectroscopy sensitivity into the infrared range, we have obtained accurate measurements of the band structures along the high-symmetry directions (X-W-K-L-U) of polymeric three-dimensional, rod-connected diamond photonic crystals. Our implementation also allows us to record single-wavelength reflectance far-field patterns showing very good agreement with simulations of the same designs.
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