Exciton-polaritons are mutually interacting quantum hybridizations of confined photons and electronic excitations. Here, we demonstrate a system of optically guided, electrically polarized exciton-polaritons ("dipolaritons") that displays up to 200-fold enhancement of the polariton-polariton interaction strength compared to unpolarized polaritons. The magnitude of the dipolar interaction enhancement can be turned on and off and can be easily tuned over a very wide range by varying the applied polarizing electric field. The large interaction strengths and the very long propagation distances of these fully guided dipolaritons open up new opportunities for realizing complex quantum circuitry and quantum simulators, as well as topological states based on exciton-polaritons, for which the interactions between polaritons need to be large and spatially or temporally controlled. The results also raise fundamental questions on the origin of these large enhancements.
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http://dx.doi.org/10.1126/sciadv.aat8880 | DOI Listing |
Nat Commun
June 2023
Department of Physics and Astronomy, The University of Sheffield, Sheffield, S3 7RH, UK.
Nonlinear interactions between excitons strongly coupled to light are key for accessing quantum many-body phenomena in polariton systems. Atomically-thin two-dimensional semiconductors provide an attractive platform for strong light-matter coupling owing to many controllable excitonic degrees of freedom. Among these, the recently emerged exciton hybridization opens access to unexplored excitonic species, with a promise of enhanced interactions.
View Article and Find Full Text PDFNat Commun
October 2022
Department of Physics, City College of New York, New York, NY, USA.
Realizing nonlinear optical response in the low photon density limit in solid-state systems has been a long-standing challenge. Semiconductor microcavities in the strong coupling regime hosting exciton-polaritons have emerged as attractive candidates in this context. However, the weak interaction between these quasiparticles has been a hurdle in this quest.
View Article and Find Full Text PDFPhys Rev Lett
November 2018
Institute of Quantum Electronics, ETH Zurich, CH-8093 Zurich, Switzerland.
Nonperturbative coupling between cavity photons and excitons leads to the formation of hybrid light-matter excitations, termed polaritons. In structures where photon absorption leads to the creation of excitons with aligned permanent dipoles, the elementary excitations, termed dipolar polaritons, are expected to exhibit enhanced interactions. Here, we report a substantial increase in interaction strength between dipolar polaritons as the size of the dipole is increased by tuning the applied gate voltage.
View Article and Find Full Text PDFSci Adv
October 2018
Racah Institute of Physics, The Hebrew University of Jerusalem, Jerusalem 91904, Israel.
Exciton-polaritons are mutually interacting quantum hybridizations of confined photons and electronic excitations. Here, we demonstrate a system of optically guided, electrically polarized exciton-polaritons ("dipolaritons") that displays up to 200-fold enhancement of the polariton-polariton interaction strength compared to unpolarized polaritons. The magnitude of the dipolar interaction enhancement can be turned on and off and can be easily tuned over a very wide range by varying the applied polarizing electric field.
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