A mixed-ion strategy to construct CNT-decorated Co/N-doped hollow carbon for enhanced oxygen reduction.

Chem Commun (Camb)

Department of Chemistry, Renmin University of China, Beijing 100872, P. R. China.

Published: October 2018

AI Article Synopsis

  • A new method is introduced for creating carbon nanotube-decorated Co/N-doped hollow carbon hybrids using a mixed-ion strategy by adjusting the Co2+/Zn2+ ratio in ZIFs-CoxZn1-x precursors.
  • The resulting catalyst, CNTs-Co/NHC-0.23, exhibits exceptional catalytic performance and longevity in the oxygen reduction reaction (ORR).
  • It outperforms commercial platinum-carbon (Pt/C) catalysts, indicating its potential for better efficiency in applications.

Article Abstract

A mixed-ion strategy to achieve carbon nanotube-decorated Co/N-doped hollow carbon hybrids (CNTs-Co/NHC) is developed by precisely controlling the Co2+/Zn2+ molar ratio in the ZIFs-CoxZn1-x precursor. The optimized CNTs-Co/NHC-0.23 catalyst shows outstanding catalytic activity and durability for the oxygen reduction reaction (ORR) and outperformed commercial Pt/C.

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http://dx.doi.org/10.1039/c8cc05959dDOI Listing

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