Enhanced superconductivity of BaKFeAs under surface potassium dosing.

J Phys Condens Matter

State Key Laboratory of Surface Physics, Department of Physics, and Laboratory of Advanced Materials, Fudan University, Shanghai 200433, People's Republic of China. Collaborative Innovation Center of Advanced Microstructures, Nanjing 210093, People's Republic of China.

Published: November 2018

Surface potassium dosing has been proven to be an effective method in tuning the electron doping and enhancing the superconducting transition temperatures in both iron chalcogenides and electron doped iron pnictides. However, it is not clear how surface potassium dosing affects the hole doping and superconductivity in hole doped Fe-based superconductors. Here we performed K-dosing on BaKFeAs, a prototypical hole-doped iron pnictide compound, and explored the electronic structure by in situ angle-resolved photoemission spectroscopy measurements. Starting from the slightly over-doped BaKFeAs, surface K-dosing effectively reduces the hole concentration towards optimal doping and enhances the superconductivity. Intriguingly, the enhancement of superconductivity does not slow down at optimal doping, and the gap further increases with K dosing even when the carrier doping effect is saturated. Meanwhile, the quasiparticle coherence of the inner hole pockets is enhanced by higher K dosing. Our results uncover a novel scattering-reduction effect of K-dosing in Ba K FeAs, which collaborates with the carrier doping effect and enhances superconductivity.

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http://dx.doi.org/10.1088/1361-648X/aae423DOI Listing

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