The ability to detect and distinguish quantum interference signatures is important for both fundamental research and for the realization of devices such as electron resonators, interferometers and interference-based spin filters. Consistent with the principles of subwavelength optics, the wave nature of electrons can give rise to various types of interference effects, such as Fabry-Pérot resonances, Fano resonances and the Aharonov-Bohm effect. Quantum interference conductance oscillations have, indeed, been predicted for multiwall carbon nanotube shuttles and telescopes, and arise from atomic-scale displacements between the inner and outer tubes. Previous theoretical work on graphene bilayers indicates that these systems may display similar interference features as a function of the relative position of the two sheets. Experimental verification is, however, still lacking. Graphene nanoconstrictions represent an ideal model system to study quantum transport phenomena due to the electronic coherence and the transverse confinement of the carriers. Here, we demonstrate the fabrication of bowtie-shaped nanoconstrictions with mechanically controlled break junctions made from a single layer of graphene. Their electrical conductance displays pronounced oscillations at room temperature, with amplitudes that modulate over an order of magnitude as a function of subnanometre displacements. Surprisingly, the oscillations exhibit a period larger than the graphene lattice constant. Charge-transport calculations show that the periodicity originates from a combination of the quantum interference and lattice commensuration effects of two graphene layers that slide across each other. Our results provide direct experimental observation of a Fabry-Pérot-like interference of electron waves that are partially reflected and/or transmitted at the edges of the graphene bilayer overlap region.
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http://dx.doi.org/10.1038/s41565-018-0258-0 | DOI Listing |
J Hazard Mater
January 2025
Henan Collaborative Innovation Center of Environmental Pollution Control and Ecological Restoration, School of Materials and Chemical Engineering, Zhengzhou University of Light Industry, Zhengzhou 450001, China.
Ibuprofen (IBU), a commonly used non-steroidal anti-inflammatory drug, is frequently detected in wastewater treatment systems, where it can interfere with nitrogen removal. This study investigated the effects of IBU on nitrogen removal performance and its biotransformation in a coupled sulfur autotrophic denitrification and anammox (SAD/A) system. Moreover, key parameters, such as nitrogen removal efficiency, microbial activity, community structure, and IBU degradation products, were carefully monitored.
View Article and Find Full Text PDFNat Nanotechnol
January 2025
Bay Area Center for Electron Microscopy, Songshan Lake Materials Laboratory, Dongguan, China.
Skyrmions can form regular arrangements, so-called skyrmion crystals (SkXs). A mode with multiple wavevectors q then describes the arrangement. While magnetic SkXs, which can emerge in the presence of Dzyaloshinskii-Moriya interaction, are well established, polar skyrmion lattices are still elusive.
View Article and Find Full Text PDFBiomed Opt Express
January 2025
State Key Laboratory of Advanced Optical Communication Systems and Networks, School of Electronics, and Center for Quantum Information Technology, Peking University, Beijing 100871, China.
Optically-pumped magnetometer (OPM) has been of increasing interest for biomagnetic measurements due to its low cost and portability compared with superconducting quantum interference devices (SQUID). Miniaturized spin-exchange-relaxation-free (SERF) OPMs typically have limited bandwidth (less than a few hundred Hertz), making it difficult to measure high-frequency biomagnetic signals such as the magnetocardiography (MCG) signal of the mouse. Existing experiments mainly use SQUID systems to measure the signal.
View Article and Find Full Text PDFQuantum backflow (QB), a counterintuitive interference phenomenon where particles with positive momentum can propagate backward, is important in applications involving light-matter interactions. To date, experimental demonstrations of backflow have been restricted to classical optical systems using techniques such as slit scanning or Shack-Hartmann wavefront sensing, which suffer from low spatial resolution due to the inherent limitations in slit width and lenslet array density. Here, we report an observation of azimuthal backflow (AB) both theoretically and experimentally by employing the weak measurement technique, which enables the precise extraction of photon momentum at each pixel.
View Article and Find Full Text PDFChemistry
December 2024
School of Materials Science and Technology, China University of Geosciences, Beijing, 10083, China.
Investigating the correlation between metal coordination and molecular conductivity in single-molecule systems is essential for advancing our knowledge of molecular electronics, particularly in the realm of spintronics. In the present study, we developed two complex wires utilizing the bipyridine ligand and two transition metal ions, Co and Zn, aiming to study the impact of different spin characters on single-molecule charge transport properties. Single-molecule conductance was investigated using scanning tunnelling microscope breaking junctions (STM-BJ) technique and the underlying mechanism was analysed by density functional theory (DFT) calculations.
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