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Global Sources of Fine Particulate Matter: Interpretation of PM Chemical Composition Observed by SPARTAN using a Global Chemical Transport Model. | LitMetric

AI Article Synopsis

Article Abstract

Exposure to ambient fine particulate matter (PM) is a leading risk factor for the global burden of disease. However, uncertainty remains about PM sources. We use a global chemical transport model (GEOS-Chem) simulation for 2014, constrained by satellite-based estimates of PM to interpret globally dispersed PM mass and composition measurements from the ground-based surface particulate matter network (SPARTAN). Measured site mean PM composition varies substantially for secondary inorganic aerosols (2.4-19.7 μg/m), mineral dust (1.9-14.7 μg/m), residual/organic matter (2.1-40.2 μg/m), and black carbon (1.0-7.3 μg/m). Interpretation of these measurements with the GEOS-Chem model yields insight into sources affecting each site. Globally, combustion sectors such as residential energy use (7.9 μg/m), industry (6.5 μg/m), and power generation (5.6 μg/m) are leading sources of outdoor global population-weighted PM concentrations. Global population-weighted organic mass is driven by the residential energy sector (64%) whereas population-weighted secondary inorganic concentrations arise primarily from industry (33%) and power generation (32%). Simulation-measurement biases for ammonium nitrate and dust identify uncertainty in agricultural and crustal sources. Interpretation of initial PM mass and composition measurements from SPARTAN with the GEOS-Chem model constrained by satellite-based PM provides insight into sources and processes that influence the global spatial variation in PM composition.

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http://dx.doi.org/10.1021/acs.est.8b01658DOI Listing

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