Spin dynamics of the block orbital-selective Mott phase.

Nat Commun

Department of Physics and Astronomy, University of Tennessee, Knoxville, TN, 37996, USA.

Published: September 2018

Iron-based superconductors display a variety of magnetic phases originating in the competition between electronic, orbital, and spin degrees of freedom. Previous theoretical investigations of the multi-orbital Hubbard model in one-dimension revealed the existence of an orbital-selective Mott phase (OSMP) with block spin order. Recent inelastic neutron scattering (INS) experiments on the BaFeSe ladder compound confirmed the relevance of the block-OSMP. Moreover, the powder INS spectrum revealed an unexpected structure, containing both low-energy acoustic and high-energy optical modes. Here we present the theoretical prediction for the dynamical spin structure factor within a block-OSMP regime using the density-matrix renormalization-group method. In agreement with experiments, we find two dominant features: low-energy dispersive and high-energy dispersionless modes. We argue that the former represents the spin-wave-like dynamics of the block ferromagnetic islands, while the latter is attributed to a novel type of local on-site spin excitations controlled by the Hund coupling.

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http://www.ncbi.nlm.nih.gov/pmc/articles/PMC6137186PMC
http://dx.doi.org/10.1038/s41467-018-06181-6DOI Listing

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