The performance of ultrafast time-stretch imaging at long wavelengths (beyond 1.5 μm) has suffered from low detection sensitivity due to the increasing loss of optical dispersive fibers. Here, we report an ultrafast optical imaging system with a line scan rate of ∼19 MHz at the 2.0-μm wavelength window by combining second-harmonic generation (SHG) with the highly sensitive time-stretch detection at 1.0 μm. In this imaging system, the sample is illuminated by the pulsed laser source at 2.0 μm in the spectrally encoding manner. After SHG, the encoded spectral signal at 2.0 μm is converted to 1.0 μm and then mapped to the time domain through a highly dispersive fiber at 1.0 μm, which provides a superior dispersion-to-loss ratio of ∼53 ps/nm/dB, ∼50 times larger than that of the standard fibers at 2.0 μm (typically ∼1.1 ps/nm/dB). These efforts make it possible for time-stretch technology not only being translated to longer wavelengths, where unique optical absorption contrast exists, but also benefitting from the high detection sensitivity at shorter wavelengths.
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http://dx.doi.org/10.1364/OL.43.003822 | DOI Listing |
J Chem Theory Comput
January 2025
State Key Laboratory for Mesoscopic Physics and Collaborative Innovation Center of Quantum Matter, School of Physics, Peking University, Beijing 100871, China.
With the advancement of high harmonic generation and X-ray free-electron lasers (XFELs) to the attosecond domain, the studies of the ultrafast electron and spin dynamics became possible. Yet, the methods for efficient control and measurement of the quantum state are to be further developed. In this publication, we propose using magnetic X-ray scattering (MXS) for resolving the molecular spin-state dynamics and establish a complete protocol to simulate MXS diffraction patterns in molecules with ab initio quantum chemistry based on the multiconfigurational method.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
College of Optical, Mechanical and Electrical Engineering, Zhejiang A&F University, Lin'an 311300, China.
As a member of the chalcogenide family, NiSe exhibits a direct bandgap of 1.74 eV, making it a promising candidate for nonlinear optical devices. However, its potential in the near-infrared region of the telecommunication band has not been fully explored.
View Article and Find Full Text PDFAdv Mater
December 2024
Institute of Frontier & Interdisciplinary Science, Shandong University, Qingdao, 266237, China.
Electrochromism stands out as a highly promising technology for applications including variable optical attenuators, optical switches, transparent displays, and dynamic windows. The pursuit of high-contrast tunability in electrochromic devices remains a challenging goal. Here, the first photochromic hydrogel electrolyte is reported for electro- and photo-dual responsive chromatic devices that yield a high transmittance contrast at 633 nm (ΔT = 83.
View Article and Find Full Text PDFNat Commun
December 2024
Department of Electronic Engineering, The Chinese University of Hong Kong, Shatin, Hong Kong SAR, China.
Reservoir computing (RC) is a powerful machine learning algorithm for information processing. Despite numerous optical implementations, its speed and scalability remain limited by the need to establish recurrent connections and achieve efficient optical nonlinearities. This work proposes a streamlined photonic RC design based on a new paradigm, called next-generation RC, which overcomes these limitations.
View Article and Find Full Text PDFNat Commun
December 2024
Department of Physics and Astronomy, Seoul National University, Seoul, 08826, Korea.
Fermi polarons are emerging quasiparticles when a bosonic impurity immersed in a fermionic bath. Depending on the boson-fermion interaction strength, the Fermi-polaron resonances exhibit either attractive or repulsive interactions, which impose further experimental challenges on understanding the subtle light-driven dynamics. Here, we report the light-driven dynamics of attractive and repulsive Fermi polarons in monolayer WSe devices.
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