Chem Commun (Camb)
Graduate School of Engineering, Osaka University, 2-1 Yamadaoka, Suita, Osaka 565-0871, Japan.
Published: August 2018
Photocatalytic H2O2 production via two-electron reduction of O2 was realized by visible-light irradiation of a metal-organic framework, MIL-125-NH2, in the presence of TEOA and benzylalcohol. Deposition of NiO nanoparticles onto MIL-125-NH2 dramatically enhanced the catalytic activity. Further studies suggested that fast disproportionation of the O2˙- intermediate to H2O2 resulted in the enhancement.
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http://dx.doi.org/10.1039/c8cc02679c | DOI Listing |
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