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Thermoresponsive Amphoteric Metal-Organic Frameworks for Efficient and Reversible Adsorption of Multiple Salts from Water. | LitMetric

AI Article Synopsis

  • Researchers developed a novel thermoresponsive metal-organic framework (MOF) that can effectively absorb various salts from saline water at room temperature and release them at higher temperatures (like 80 °C).
  • The MOF, which integrates cation- and anion-binding functionalities through the introduction of a polymer, demonstrates impressive salt adsorption abilities with high capacities for salts like LiCl and NaCl.
  • This advancement offers an innovative and eco-friendly approach to creating materials for enhanced water desalination and purification processes.

Article Abstract

Regenerable, high-efficiency salt sorption materials are highly desirable for water treatment. Here, a thermoresponsive, amphoteric metal-organic framework (MOF) material is reported that can adsorb multiple salts from saline water at room temperature and effectively release the adsorbed salts into water at elevated temperature (e.g., 80 °C). The amphoteric MOF, integrated with both cation-binding carboxylic groups and anion-binding tertiary amine groups, is synthesized by introducing a polymer with tertiary amine groups into the cavities of a water-stable MOF such as MIL-121 with carboxylic groups inside its frameworks. The amphoterized MIL-121 exhibits excellent salt adsorption properties, showing stable adsorption-desorption cycling performances and high LiCl, NaCl, MgCl , and CaCl adsorption capacities of 0.56, 0.92, 0.25, and 0.39 mmol g , respectively. This work provides a novel, effective strategy for synthesizing new-generation, environmental-friendly, and responsive salt adsorption materials for efficient water desalination and purification.

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Source
http://dx.doi.org/10.1002/adma.201802767DOI Listing

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