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Architecting Ultra-Robust Zr(IV) Metal-Organic Framework for Energy-Efficient Desiccant Air Conditioning.
J Am Chem Soc
December 2024
School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, China.
Air-conditioning systems, composed mainly of humidity control and heat reallocation units, play a pivotal role in upholding superior air quality and human well-being across diverse environments ranging from international space stations and pharmacies to granaries and cultural relic preservation sites, and to commercial and residential buildings. The adoption of sorbent water as the working pair and low-grade renewable or waste heat in adsorption-driven air-conditioning presents a state-of-the-art solution, notably for its energy efficiency and eco-friendliness vis-à-vis conventional electricity-driven vapor compression cycles. Here, we introduce a rational π-extension strategy to engineer an ultrarobust and highly porous zirconium metal-organic framework (Zr-MOF).
View Article and Find Full Text PDFEnriched Molecular-Level View of Saline Wetland Soil Carbon by Sensitivity-Enhanced Solid-State NMR.
J Am Chem Soc
December 2024
Department of Chemistry, Michigan State University, East Lansing, Michigan 48824, United States.
Article Synopsis
- Soil organic matter (SOM) is crucial for reducing greenhouse gas emissions and supporting global climate, carbon cycles, and biodiversity.
- Coastal wetland soils, which constitute one-third of SOM, are eroding rapidly due to rising sea levels, highlighting a gap in research on carbon sequestration in these areas compared to upland soils.
- Using solid-state nuclear magnetic resonance (ssNMR), the study reveals that some molecular structures in wetland soils have been preserved for over 1,000 years, but these structures are declining in abundance as decomposition and repolymerization processes occur, making coastal wetland SOM increasingly vulnerable to environmental changes.
Seasonal changes in pigment content in overwintering and current-year leaves of Sasa senanensis from snowmelt to before leaf-fall of canopy deciduous trees.
J Plant Res
December 2024
Institute of Low Temperature Science, Hokkaido University, Sapporo, Hokkaido, Japan.
Sasa senanensis (a dwarf bamboo), an evergreen herbaceous plant native to the cool temperate regions of eastern Asia, endures seasonal temperature fluctuations and significant variations in light intensity typical for understory plants. Following snowmelt in early spring, the light intensity received by Sasa leaves surges, then diminishes as the canopy of upper deciduous trees develops. The current-year leaves of S.
View Article and Find Full Text PDFTruxillic calcium supramolecular skeleton fortified pH responsive and biodegradable alginate hydrogel films promoting fruit preservation.
Int J Biol Macromol
December 2024
School of Pharmaceutical Sciences, Jilin University, Changchun, Jilin 130021, China. Electronic address:
Article Synopsis
- The study developed an innovative alginate hydrogel film enhanced with a truxillic calcium skeleton, showing significant improvements in its physical and mechanical properties, making it suitable for fruit preservation.
- The best-performing film, CBDA-10-Ca/SA, can block over 50% of UV-visible light, exhibits high breaking strength (79 MPa), and shows remarkable pH responsiveness with water absorption rates ranging from 3480% to 9520%.
- All films degraded by about 70% after four weeks in soil, suggesting that polyphenols not only enhance mechanical strength but also contribute antibacterial and antioxidant properties that boost the film’s functionality.
Care in the era of digital health: experiences from Norwegian general practitioners.
Scand J Prim Health Care
December 2024
Department of Caring and Ethics, Faculty of Health Sciences, University of Stavanger, Stavanger, Norway.
Objective: This study explores the experiences of General Practitioners (GPs) in Norway, examining the role of care in their practice and the impact of digital health technologies on their caregiving approach.
Design: A qualitative study employing semi-structured interviews. The data was analysed by systematic text condensation.
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