In this work the thermoelectric generator (TEG) based on catalytic combustion already developed in our lab has been further investigated and improved. The system made of two thermoelectric (TE) modules coupled with a catalytic combustor has been used in this work to obtain higher overall efficiency by adding hydrogen to the fuel mixture. Since implementation of hydrogen as a fuel has shown low and stable combustion temperature in literature, it is expected to achieve good overall efficiency of TEG. Moreover, hydrogen can be used to improve the system inducing self-ignition. Focus of the present work is the implementation of different mixture proportions, varying the amount of hydrogen, and the investigation of their effects on the overall efficiency. The overall TEG efficiency, has been evaluated by parallel characterization of thermoelectric modules and exhaust gases composition. The system performances have been characterized using different mixtures: the results indicate that addition of H₂ to the fuel contribute to increase the chemical and overall TEG efficiency respect to previous work, producing up to 5.92 W of electrical power. Finally, the effects of H₂ for on self-ignition conditions have been investigated finding the minimum H₂ amount for different gas flow rates.
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http://dx.doi.org/10.1166/jnn.2017.13731 | DOI Listing |
Materials (Basel)
January 2025
Department of Polymer Engineering, Pukyong National University, Busan 48513, Republic of Korea.
Carbon nanotubes (CNTs) have drawn great attention as promising candidates for realizing next-generation printed thermoelectrics (TEs). However, the dispersion instability and resulting poor printability of CNTs have been major issues for their practical processing and device applications. In this work, we investigated the TE characteristics of water-processable carboxymethyl cellulose (CMC) and single-walled CNT (SWCNT) composite.
View Article and Find Full Text PDFHeliyon
January 2025
Department of Environmental Science & Engineering, Ewha Womans University, South Korea.
A path to carbon neutrality requires the development of refrigeration units that use no refrigerant or emit less greenhouse gas (GHG), such as Thermoelectric coolers (TECs). Using the life cycle inventory assessment (LCIA), the environmental impacts of the manufacturing process of TECs were analyzed, including greenhouse gas emissions, human carcinogenic toxicity (HCT), terrestrial ecotoxicity (TE), freshwater ecotoxicity (FE), mineral resource scarcity (MRS), and fossil resource scarcity (FRS). The alumina plate manufacturing process produces the most GHG emissions because it uses a lot of electricity in the sintering process.
View Article and Find Full Text PDFNanoscale
January 2025
Department of Chemical and Biomolecular Engineering, College of Design and Engineering, National University of Singapore, 117585, Singapore.
Bioelectronic devices with medical functions have attracted widespread attention in recent years. Power supplies are crucial components in these devices, which ensure their stable operation. Biomedical devices that utilize external power supplies and extended electrical wires limit patient mobility and increase the risk of discomfort and infection.
View Article and Find Full Text PDFAdv Sci (Weinh)
January 2025
Department of Materials Engineering, KU Leuven, Kasteelpark Arenberg 44, Leuven, 3001, Belgium.
The next generation of soft electronics will expand to the third dimension. This will require the integration of mechanically compliant 3D functional structures with stretchable materials. Here, omnidirectional direct ink writing (DIW) of poly(3,4-ethylenedioxythiophene): polystyrene sulfonate (PEDOT:PSS) aerogels with tunable electrical and mechanical performance is demonstrated, which can be integrated with soft substrates.
View Article and Find Full Text PDFAdv Sci (Weinh)
January 2025
SKKU Advanced Institute of Nanotechnology (SAINT) and Department of Nano Science and Technology, Sungkyunkwan University, Suwon, 16419, Republic of Korea.
A novel additive method to boost the Seebeck coefficient of doped conjugated polymers without a significant loss in electrical conductivity is demonstrated. Perovskite (CsPbBr) quantum dots (QDs) passivated by ligands with long alkyl chains are mixed with a conjugated polymer in a solution phase to form polymer-QD blend films. Solution sequential doping of the blend film with AuCl solution not only doped the conjugated polymer but also decomposed the QDs, resulting in a doped conjugated polymer film embedded with separated ions dissociated from the QDs.
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