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Research on Three-level Enrichment Method Based on 222Rn.

Health Phys

January 2023

School of Nuclear Science and Technology, University of South China, Hunan 421001, China.

Various low-concentration inert gases, including 222Rn, 133Xe, and 85Kr, pollute the atmosphere near nuclear facilities (e.g., nuclear power plants or reprocessing plants).

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Radioxenon can be produced with a high fission yield during a nuclear explosion, making it an important tracer to demonstrate the nuclear origin of an explosion. For this reason, it is continuously monitored by the Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO) as part of the verification regime. Radioxenon is emitted by civil nuclear facilities, like nuclear power plants (NPPs) or isotope production facilities (IPFs), providing significant but variable contribution to the noble gas background.

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In 2015 and 2016, atmospheric transport modeling challenges were conducted in the context of the Comprehensive Nuclear-Test-Ban Treaty (CTBT) verification, however, with a more limited scope with respect to emission inventories, simulation period and number of relevant samples (i.e., those above the Minimum Detectable Concentration (MDC)) involved.

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Positron emission tomography (PET) uses radioactive tracers and enables the functional imaging of several metabolic processes, blood flow measurements, regional chemical composition, and/or chemical absorption. Depending on the targeted processes within the living organism, different tracers are used for various medical conditions, such as cancer, particular brain pathologies, cardiac events, and bone lesions, where the most commonly used tracers are radiolabeled with 18F (e.g.

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During a nuclear accident, estimating the source terms using environmental measurements is vital for emergency decision-making. In this study, we propose a forecasting model based on a temporal convolutional network to estimate the release rates of seven radionuclides (Kr-88, Te-132, I-131, Xe-133, Cs-137, Ba-140, and Ce-144) based on off-site sequential gamma dose rates and meteorological monitoring data. To determine the best structure of the neural network, Bayesian optimization and hyperband (BOHB) was used on the hyperparameters of the model to reduce the testing loss.

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