In this work, the existence and propagation of acoustic Tamm states at the interface of air and a face-centered cubic solid-fluid phononic crystal composed of spherical air voids interconnected by cylindrical air channels are demonstrated. Supercell band structure computations via the finite element method reveal surface bands for Tamm states on (100), (110), and (111) surfaces of the phononic crystal. The states decay sharply into the phononic crystal so that only a two-row slab is sufficient to guide them over the respective surfaces without leakage, as confirmed by finite element simulations. In addition, surface wave propagation along the [10] direction of the (100) surface is experimentally demonstrated. Ability to confine the Tamm states in all three dimensions is a key aspect in designing few-layer-thick acoustic circuits. Low material filling fraction of the phononic crystal could be leveraged to realize lightweight all-acoustic systems where either bulk or surface states can be incorporated.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1121/1.5023334 | DOI Listing |
Sci Rep
January 2025
Physics Department, Faculty of Science, Beni-Suef University, Beni-Suef, 62512, Egypt.
This paper presents a novel investigation of a magnetic sensor that employs Fano/Tamm resonance within the photonic band gap of a one-dimensional crystal structure. The design incorporates a thin layer of gold (Au) alongside a periodic arrangement of Tantalum pentoxide ([Formula: see text]) and Cesium iodide ([Formula: see text]) in the configuration [Formula: see text]. We utilized the transfer matrix method in conjunction with the Drude model to analyze the formation of Fano/Tamm states and the permittivity of the metallic layer, respectively.
View Article and Find Full Text PDFJ Phys Chem Lett
January 2025
Department of Physics, Rutgers University, Newark 07102, New Jersey, United States.
A striking example of the need to accurately capture states of double-excitation character in molecules is seen in predicting photoinduced dynamics in small polyenes. Due to the coupling of electronic and nuclear motions, the dark 2Ag state, known to have double-excitation character, can be reached after an initial photoexcitation to the bright 1Bu state via crossings of their potential energy surfaces. However, the shapes of the surfaces are so poorly captured by most electronic structure methods, that the crossing is missed or substantially mis-located.
View Article and Find Full Text PDFNanoscale
January 2025
School of Physics and Optoelectronic Engineering, Beijing University of Technology, Beijing 100124, P. R. China.
Photonic crystals (PC) play a key role in optical field modulation due to their unique photonic band gaps (PBGs). Anodic aluminum oxide (AAO) prepared by pulse anodization is a promising candidate for PC devices. In this research, an AAO-based PC with multi-band was fabricated on a single-slice & single-material film, which exhibits multi-band responses in the visible-to-near-infrared (vis-NIR) region.
View Article and Find Full Text PDFJ Chem Phys
January 2025
Key Laboratory of Theoretical and Computational Photochemistry, Ministry of Education, College of Chemistry, Beijing Normal University, Beijing 100875, China.
This study presents an efficient methodology for simulating nonadiabatic dynamics of complex materials with excitonic effects by integrating machine learning (ML) models with simplified Tamm-Dancoff approximation (sTDA) calculations. By leveraging ML models, we accurately predict ground-state wavefunctions using unconverged Kohn-Sham (KS) Hamiltonians. These ML-predicted KS Hamiltonians are then employed for sTDA-based excited-state calculations (sTDA/ML).
View Article and Find Full Text PDFJ Am Chem Soc
January 2025
Institute of Molecular Physiology, Shenzhen Bay Laboratory, Shenzhen 518132, China.
Small-molecule fluorophores are invaluable tools for fluorescence imaging. However, means for their covalent conjugation to the target proteins limit applications in multicolor imaging. Here, we identify 2-[(alkylhio)(ryl)ethylene]alononitrile (TAMM) molecules reacting with 1,2-aminothiol at a labeling rate over 10 M s through detailed mechanistic investigation.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!