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| http://dx.doi.org/10.1159/000485867 | DOI Listing |
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High Performance Star Block Aliphatic Polyester Thermoplastic Elastomers Using PDLA--PLLA Stereoblock Hard Domains.
ACS Macro Lett
October 2023
Department of Chemistry, University of Minnesota, Minneapolis, Minnesota 55455-0431, United States of America.
Star block (ABC) terpolymers consisting of a rubbery poly(γ-methyl-ε-caprolactone) (PγMCL) (C) core and hard poly(l-lactide) (PLLA) (B) and poly(d-lactide) (PDLA) (A) end-blocks with varying PDLA to PLLA block ratios were explored as high-performance, sustainable, aliphatic polyester thermoplastic elastomers (APTPEs). The stereocomplexation of the PDLA/PLLA blocks within the hard domains provided the APTPEs with enhanced thermal stability and an increased resistance to permanent deformation compared to nonstereocomplex analogs. Variations in the PDLA:PLLA block ratio yielded tunable mechanical properties likely due to differences in the extent and location of stereocomplex crystallite formation as a result of architectural constraints.
View Article and Find Full Text PDFHighlights from ABC4 - Bridging the Gap.
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Li Ka Shing Faculty of Medicine, The University of Hong Kong, Hong Kong Breast Oncology Group (HKBOG), Hong Kong, Hong Kong.
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