We present a magnetic phase diagram of rare-earth pyrochlore Yb_{2}Ti_{2}O_{7} in a ⟨111⟩ magnetic field. Using heat capacity, magnetization, and neutron scattering data, we show an unusual field dependence of a first-order phase boundary, wherein a small applied field increases the ordering temperature. The zero-field ground state has ferromagnetic domains, while the spins polarize along ⟨111⟩ above 0.65 T. A classical Monte Carlo analysis of published Hamiltonians does account for the critical field in the low T limit. However, this analysis fails to account for the large bulge in the reentrant phase diagram, suggesting that either long-range interactions or quantum fluctuations govern low field properties.
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http://dx.doi.org/10.1103/PhysRevLett.119.127201 | DOI Listing |
J Phys Condens Matter
January 2025
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, No.8 South Third Street, Zhongguancun, Beijing, 100190, CHINA.
We systematically investigate the magnetization and thermodynamic responses associated with antiferromagnetic (AFM) transitions in single crystals of the magnetic semiconductor Eu3InAs3. The linear thermal expansion measurements around the AFM transition temperatures, TN1 and TN2, indicate an expansion along the a axis and contraction along the b and c axes. The calculated ∆V/V(T) shows a continuous change at TN, indicating a second-order magnetic phase transition.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
School of Energy and Power Engineering, Huazhong University of Science & Technology, Wuhan, Hubei 430074, China.
All-solid-state lithium metal batteries hold promise for meeting the industrial demands for high energy density and safety. However, voids are formed at the lithium metal anode/solid-state electrolyte interface during stripping, deteriorating interface contact and reducing the cycle stability. Stack pressure and operating temperature are effective methods to activate creep deformation in lithium metal, promoting interfacial deformation and alleviating void-induced interface issues.
View Article and Find Full Text PDFCryobiology
January 2025
Specialized Surgical Hospital "Doctor Malinov", 46, Gotse Delchev blvd., 1860 Sofia, Bulgaria.
The cryopreservation of human spermatozoa is an integral part of cryobiology, aiming to support the in-vitro fertilization. The latter relies on the availability of as much as possible reproductively active spermatozoa, whose number after thawing decreases due to the accompanied freezing injury and the cytotoxicity of cryoprotectants. An innovative option to circumvent these obstacles is to make the freezing interface non-wettable, by coating it with rapeseed oil soot possessing intrinsic cryoprotective properties, delaying the ice formation and possibly providing identical rates of intracellular dehydration and extracellular crystallization.
View Article and Find Full Text PDFNat Commun
January 2025
Center for High Pressure Science and Technology Advanced Research, Beijing, 100093, China.
Due to the sulfur's atoms' propensity to form molecules and/or polymeric chains of various sizes and configuration, elemental sulfur possesses more allotropes and polymorphs than any other element at ambient conditions. This variability of the starting building blocks is partially responsible for its rich and fascinating phase diagram, with pressure and temperature changing the states of sulfur from insulating molecular rings and chains to semiconducting low- and high-density amorphous configurations to incommensurate superconducting metallic atomic phase. Here, using a fast compression technique, we demonstrate that the rapid pressurisation of liquid sulfur can effectively break the molecular ring structure, forming a glassy polymeric state of pure-chain molecules (Am-S).
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Initiative for the Theoretical Sciences and CUNY-Princeton Center for the Physics of Biological Function, The Graduate Center, CUNY, New York, New York 10016, USA.
The random-energy model (REM), a solvable spin-glass model, has impacted an incredibly diverse set of problems, from protein folding to combinatorial optimization, to many-body localization. Here, we explore a new connection to secret sharing. We derive an analytic expression for the mutual information between any two disjoint thermodynamic subsystems of the REM.
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