Magnetic Excitations and Continuum of a Possibly Field-Induced Quantum Spin Liquid in α-RuCl_{3}.

Phys Rev Lett

Experimental Physics V, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, 86135 Augsburg, Germany.

Published: December 2017

We report on terahertz spectroscopy of quantum spin dynamics in α-RuCl_{3}, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. We follow the evolution of an extended magnetic continuum below the structural phase transition at T_{s2}=62  K. With the onset of a long-range magnetic order at T_{N}=6.5  K, spectral weight is transferred to a well-defined magnetic excitation at ℏω_{1}=2.48  meV, which is accompanied by a higher-energy band at ℏω_{2}=6.48  meV. Both excitations soften in a magnetic field, signaling a quantum phase transition close to B_{c}=7  T, where a broad continuum dominates the dynamical response. Above B_{c}, the long-range order is suppressed, and on top of the continuum, emergent magnetic excitations evolve. These excitations follow clear selection rules and exhibit distinct field dependencies, characterizing the dynamical properties of a possibly field-induced quantum spin liquid.

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http://dx.doi.org/10.1103/PhysRevLett.119.227202DOI Listing

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