α-RuCl_{3} is a leading candidate material for the observation of physics related to the Kitaev quantum spin liquid (QSL). By combined susceptibility, specific-heat, and nuclear-magnetic-resonance measurements, we demonstrate that α-RuCl_{3} undergoes a quantum phase transition to a QSL in a magnetic field of 7.5 T applied in the ab plane. We show further that this high-field QSL phase has gapless spin excitations over a field range up to 16 T. This highly unconventional result, unknown in either Heisenberg or Kitaev magnets, offers insight essential to establishing the physics of α-RuCl_{3}.
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http://dx.doi.org/10.1103/PhysRevLett.119.227208 | DOI Listing |
Phys Rev Lett
November 2024
Department of Condensed Matter Physics, Weizmann Institute of Science, Rehovot 7610001, Israel.
The Kitaev honeycomb model supports gapless and gapped quantum spin liquid phases. Its exact solvability relies on extensively many locally conserved quantities. Any real-world manifestation of these phases would include imperfections in the form of disorder and interactions that break integrability.
View Article and Find Full Text PDFPhys Chem Chem Phys
December 2024
Guizhou Provincial Key Laboratory of Computing and Network Convergence, School of Information, Guizhou University of Finance and Economics, Guiyang 550025, People's Republic of China.
The quantum spin Hall (QSH) effect has attracted extensive research interest due to its great promise in topological quantum computing and novel low-energy electronic devices. Here, using first-principles calculations, we find that MX (M = Ru and Os; X = As and Sb) monolayers are 2D topological insulators (TIs). The spin-orbit coupling (SOC) band gaps for RuAs, RuSb, OsAs, and OsSb monolayers are predicted to be 80, 131, 118, and 221 meV, respectively.
View Article and Find Full Text PDFSci Rep
December 2024
Mathematical Sciences Institute, Australian National University, Canberra, ACT, 2601, Australia.
In this study, we delve into the intricate ground state phase diagram of anisotropic spin-1/2 XXZ chains under the uniform Gamma interaction. Employing the robust infinite time evolving block decimation (iTEBD) technique and the Lanczos technique, we meticulously obtain the model's ground state properties. Complementing our numerical analysis, we derive analytical approximations through a mean-field framework, transposed into the fermionic representation.
View Article and Find Full Text PDFPhys Rev Lett
November 2024
Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA.
In the presence of an external magnetic field, the Kitaev model could host either gapped topological anyons or gapless Majorana fermions. In α-RuCl_{3}, the gapped and gapless cases are only separated by a 30° rotation of the in-plane magnetic field vector. The presence or absence of the spectral gap is key for understanding the thermal transport behavior in α-RuCl_{3}.
View Article and Find Full Text PDFPhys Chem Chem Phys
December 2024
School of Physics and Electronic Engineering, LinYi University, LinYi 276000, China.
This study employed first-principles calculations to comprehensively explore the structural, electronic, and magnetic properties of transition metal-doped biphenylene networks (BPNs). Initially, we optimized the most stable structures of biphenylene doped with various transition metals (Sc, Ti, V, Cr, Mn, Fe, Co, Ni, Cu, and Zn) and analysed their doping energies and electronic structures in detail. The results indicate that the introduction of transition metals induces varying degrees of spin polarization.
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