Ultrastrong light-matter coupling allows the exploration of new states of matter through the interaction of strong vacuum fields with huge electronic dipoles. By using hybrid dipole antenna-split ring resonator-based cavities with extremely small effective mode volumes V/λ ≃ 6 × 10 and surfaces S/λ ≃ 3.5 × 10, we probe the ultrastrong light-matter coupling at 300 GHz to less than 100 electrons located in the last occupied Landau level of a high mobility two-dimensional electron gas, measuring a normalized coupling ratio of Ω/ω = 0.36. Effects of the extremely reduced cavity dimensions are observed as the light-matter coupled system is better described by an effective mass heavier than the uncoupled one. These results open the way to ultrastrong coupling at the single-electron level in two-dimensional electron systems.
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http://dx.doi.org/10.1021/acs.nanolett.7b03228 | DOI Listing |
Nanophotonics
June 2024
Department of Chemistry and Biochemistry, University of California San Diego, La Jolla, CA 92093, USA.
The vacuum Rabi splitting (VRS) in molecular polaritons stands as a fundamental measure of collective light-matter coupling. Despite its significance, the impact of molecular disorder on VRS is not fully understood yet. This study delves into the complexities of VRS amidst various distributions and degrees of disorder.
View Article and Find Full Text PDFNanophotonics
June 2024
Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, E-28049 Madrid, Spain.
The full information about the interaction between a quantum emitter and an arbitrary electromagnetic environment is encoded in the so-called spectral density. We present an approach for describing such interaction in any coupling regime, providing a Lindblad-like master equation for the emitter dynamics when coupled to a general nanophotonic structure. Our framework is based on the splitting of the spectral density into two terms.
View Article and Find Full Text PDFACS Nano
December 2024
Department of Physics, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States.
Collective excitations of bound electron-hole pairs, i.e., excitons, are ubiquitous in condensed matter systems, and it has been shown that they can strongly couple to other degrees of freedom, such as spin, orbital, and lattice.
View Article and Find Full Text PDFNat Commun
December 2024
Humboldt Centre for Nano- and Biophotonics, Institute for Light and Matter, Department of Chemistry, University of Cologne, Greinstr. 4-6, Köln, Germany.
Thin film interference is integral to modern photonics, e.g., allowing for precise design of high performance optical filters, photovoltaics and light-emitting devices.
View Article and Find Full Text PDFJ Chem Phys
November 2024
Department of Chemistry, University of North Carolina Charlotte, 9201 University City Bldv, Charlotte, North Carolina 07470A, USA.
Molecules under strong or ultra-strong light-matter coupling present an intriguing route to modify chemical structure, properties, and reactivity. A rigorous theoretical treatment of such systems requires handling matter and photon degrees of freedom on an equal quantum mechanical footing. In the regime of molecular electronic strong or ultra-strong coupling to one or a few molecules, it is desirable to treat the molecular electronic degrees of freedom using the tools of ab initio quantum chemistry, yielding an approach referred to as ab initio cavity quantum electrodynamics (ai-QED), where the photon degrees of freedom are treated at the level of cavity QED.
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