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Lattice Distortions Promoting the In-Depth Reconstruction of Ni-Based Electrocatalysts with Enriched Oxygen Vacancies for the Electrochemical Oxidation of 5-Hydroxymethylfurfural toward 2,5-Furandicarboxylic Acid.
Inorg Chem
January 2025
Fujian Provincial Key Laboratory of Advanced Materials Oriented Chemical Engineering, College of Chemistry and Material Science, Fujian Normal University, No. 8 Shangsan Road, Fuzhou 350007, China.
The electrocatalytic 5-hydroxymethylfurfural (HMF) oxidation reaction (HMFOR) toward 2,5-furandicarboxylic acid (FDCA) has been considered a promising approach for the substitution of the energy-consuming and hazardous oxygen evolution reaction and for the valorization of renewable biomass. However, it is limited by the susceptibility of HMF to the oxidative environment and requires efficient electrocatalysts. Herein, a NiMo complex (NiMo-N) is provided as the precatalyst for the HMFOR, exhibiting favorable performances with a current density of 450 mA·cm achieved at an anodic potential of 1.
View Article and Find Full Text PDFBoosting selective chlorine evolution reaction: Impact of Ag doping in RuO electrocatalysts.
J Colloid Interface Sci
January 2025
School of Rare Earths, University of Science and Technology of China, Hefei, Anhui 230026, PR China; Key Laboratory of Rare Earths, Ganjiang Innovation Academy, Chinese Academy of Sciences, Ganzhou, Jiangxi 341000, PR China. Electronic address:
The chlor-alkali process is critical to the modern chemical industry because of the wide utilization of chlorine gas (Cl). More than 95 % of global Cl production relies on electrocatalytic chlorine evolution reaction (CER) through chlor-alkali electrolysis. The RuO electrocatalyst serves as the main active component widely used in commercial applications.
View Article and Find Full Text PDFAllostery and Evolution: A Molecular Journey Through the Structural and Dynamical Landscape of an Enzyme Super Family.
Mol Biol Evol
January 2025
Univ. Grenoble Alpes, CNRS, CEA, IBS, 38000 Grenoble, France.
Allosteric regulation is a powerful mechanism for controlling the efficiency of enzymes. Deciphering the evolutionary mechanisms by which allosteric properties have been acquired in enzymes is of fundamental importance. We used the malate (MalDH) and lactate deydrogenases (LDHs) superfamily as model to elucidate this phenomenon.
View Article and Find Full Text PDFCost-effectiveness of decentralising acute malnutrition treatment with a standard or simplified treatment protocol: an economic evaluation in the region of Gao, Mali.
BMC Public Health
January 2025
Nutrition and Health Department, Action Against Hunger, Madrid, Spain.
Background: Acute malnutrition treatment coverage remains low worldwide, causing significant morbidity and mortality. Decentralisation of treatment to Community Health Worker (CHW) sites has shown to be an effective strategy to improve access and increase coverage, but evidence on the cost and cost-effectiveness of this approach as well the use of simplified treatment protocols in conflict settings is lacking. The objective of this study was to determine cost per child treated as well as the cost-effectiveness of the hybrid model of treatment delivery (where treatment is provided at both health facilities and CHW sites) using either a standard protocol (Intervention 1) or simplified protocol (Intervention 2) compared to standard treatment at health facilities only (Control) in the conflict affected region of Gao in Northern Mali.
View Article and Find Full Text PDFRapid screening of pottery lipid residue profile via comprehensive two-dimensional gas chromatography.
Anal Chim Acta
February 2025
Department of Archaeology and Anthropology, School of Humanities, University of Chinese Academy of Sciences, 100049, Beijing, China. Electronic address:
Background: Pottery lipid residue analysis has been extensively practiced worldwide as an important part of archaeometry studies, but in some cases, the complexity of archaeological residue cannot be fully revealed by one-dimensional gas chromatography (1D GC) separation. Although the development of comprehensive two-dimensional gas chromatography (GCxGC) has offered another way to achieve better separation and higher resolution, GCxGC separation has rarely been applied to pottery residue analysis. Clearly, GCxGC separation needs to be explored to examine and scrutinize the complexity of pottery lipid residue profile as well as rapid data treatment workflow.
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