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http://dx.doi.org/10.1056/NEJMc1712990 | DOI Listing |
Natl Sci Rev
December 2024
Laboratoire des Sciences du Climat et de l'Environnement, University Paris Saclay CEA CNRS, Gif sur Yvette 91191, France.
In 2023, the CO growth rate was 3.37 ± 0.11 ppm at Mauna Loa, which was 86% above that of the previous year and hit a record high since observations began in 1958, while global fossil fuel CO emissions only increased by 0.
View Article and Find Full Text PDFNatl Sci Rev
December 2024
Institute of Carbon Neutrality, Sino-French Institute for Earth System Science, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China.
Atmospheric CO growth rate (CGR), reflecting the carbon balance between anthropogenic emissions and net uptake from land and ocean, largely determines the magnitude and speed of global warming. The CGR at Mauna Loa Baseline Observatory reached a record high in 2023. We quantified major components of the global carbon balance for 2023, by developing a framework that integrated fossil fuel CO emissions data and an atmospheric inversion from the Global ObservatioN-based system for monitoring Greenhouse GAses (GONGGA) with two artificial intelligence (AI) models derived from dynamic global vegetation models.
View Article and Find Full Text PDFNat Commun
November 2024
State Key Laboratory of Vaccines for Infectious Diseases, Center for Molecular Imaging and Translational Medicine, School of Public Health, Xiamen University, Xiamen, Fujian, China.
Constructing organic fluorophosphines, vital drug skeletons, through the direct fluorination of readily available alkyl phosphonates has been impeded due to the intrinsic low electrophilicity of P and the high bond energy of P═O bond. Here, alkyl phosphonates are electrophilically activated with triflic anhydride and N-heteroaromatic bases, enabling nucleophilic fluorination at room temperature to form fluorophosphines via reactive phosphine intermediates. This approach facilitates the late-stage (radio)fluorination of broad dialkyl and monoalkyl phosphonates.
View Article and Find Full Text PDFEnviron Int
December 2024
Institute of Environmental Assessment and Water Research (IDAEA-CSIC), 08034 Barcelona, Spain. Electronic address:
There is a body of evidence that ultrafine particles (UFP, those with diameters ≤ 100 nm) might have significant impacts on health. Accordingly, identifying sources of UFP is essential to develop abatement policies. This study focuses on urban Europe, and aims at identifying sources and quantifying their contributions to particle number size distribution (PNSD) using receptor modelling (Positive Matrix Factorization, PMF), and evaluating long-term trends of these source contributions using the non-parametric Theil-Sen's method.
View Article and Find Full Text PDFInt Angiol
August 2024
Department of Vascular Surgery, Copenhagen University Hospital Rigshospitalet, Copenhagen, Denmark.
Background: The current management of abdominal aortic aneurysm (AAA) hinges upon assessing diameter using ultrasound (US). Diameter reproducibility with conventional two-dimensional ultrasound (2D-US) is challenging and requires experienced operators. A novel automatic three-dimensional ultrasound (3D-US) system enables on-cart software-assisted diameter estimation (3D-SAUS), potentially facilitating more precise diameter measurements than 2D-US.
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