In recent years, severe haze events often occurred in China, causing serious environmental problems. The mechanisms responsible for the haze formation, however, are still not well understood, hindering the forecast and mitigation of haze pollution. Our study of the 2012-13 winter haze events in Beijing shows that atmospheric water vapour plays a critical role in enhancing the heavy haze events. Under weak solar radiation and stagnant moist meteorological conditions in winter, air pollutants and water vapour accumulate in a shallow planetary boundary layer (PBL). A positive feedback cycle is triggered resulting in the formation of heavy haze: (1) the dispersal of water vapour is constrained by the shallow PBL, leading to an increase in relative humidity (RH); (2) the high RH induces an increase of aerosol particle size by enhanced hygroscopic growth and multiphase reactions to increase particle size and mass, which results in (3) further dimming and decrease of PBL height, and thus further depressing of aerosol and water vapour in a very shallow PBL. This positive feedback constitutes a self-amplification mechanism in which water vapour leads to a trapping and massive increase of particulate matter in the near-surface air to which people are exposed with severe health hazards.
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http://dx.doi.org/10.1038/s41598-017-15909-1 | DOI Listing |
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March 2025
Engineering Laboratory for AgroBiomass Recycling & Valorizing, College of Engineering, China Agricultural University, Beijing, 100083, China.
Chemical upcycling of plastic waste to produce green H has emerged as a promising avenue. Highly efficient and robust NiAlO catalysts with dual active nanocomposite (NiO-NiAlO) through a facile electronic configuration modulation strategy are synthesized for the decomposition-catalytic steam reforming (DCSR) of plastic wastes for enhancing H production while alleviating carbon deposition. Of these dual-active nanocomposite catalysts, NiAlO-800 presents the highest proportions of Ni cations and oxygen vacancies, contributing to the enhance structural stability and catalytic activity.
View Article and Find Full Text PDFACS Electrochem
March 2025
Institute of Physical Chemistry, University of Innsbruck, Innrain 52c, A-6020 Innsbruck, Austria.
Solid oxide cell technologies play a crucial role in climate change mitigation by enabling the reversible storage of renewable energy. Understanding the electrochemical high-temperature reaction mechanisms and the catalytic role of the electrode and electrolyte materials is essential for advancing power-to-H technologies. Despite its significance, limited spectroscopic research focusing on nickel and yttria-stabilized zirconia (Ni/YSZ) is available.
View Article and Find Full Text PDFInt J Biol Macromol
March 2025
Heilongjiang Academy Of Chinese Medicine Sciences, Institute of Chinese Materia Medica, No.72, Xiang'an Street, Xiangfang District, Harbin 150036, Heilongjiang, China. Electronic address:
Polygonatum cyrtonema (PC) is a traditional Chinese herb used in both food and medicine with considerable bioactivity. The nine-steam processed pieces of PC are the main form of clinical application, while research has focused on the polysaccharide of their crude form. This study evaluated the physicochemical characteristics and protective effects of crude PC (PCP) and nine-steamed PC (NPCP) against cyclophosphamide (CTX)-induced immunosuppression.
View Article and Find Full Text PDFJ Environ Manage
March 2025
National-Local Joint Engineering Research Center of Biomass Refining and High-Quality Utilization, Changzhou Key Laboratory of Biomass Green, Safe & High Value Utilization Technology, Institute of Urban and Rural Mining, Changzhou University, Changzhou 213164, China. Electronic address:
Converting biomass waste into hydrogen energy through gasification is a crucial pathway for producing "green hydrogen". In a fixed bed reactor, a representative biomass waste, rice straw (RS), was pyrolyzed at N, HO, CO, and O atmospheres to generate hydrogen. Solid C-13 Nuclear Magnetic Resonance Spectroscopy (C-NMR) and Fourier Transform infrared spectroscopy (FTIR) were employed to elucidate the carbon structure and functional groups of the samples.
View Article and Find Full Text PDFJ Environ Manage
March 2025
School of Environment and Municipal Engineering, Lanzhou Jiaotong University, Lanzhou, 730070, China.
Landfill stale waste (LSW) poses considerable environmental issues, especially concerning methane emissions and the ecosystem contamination. This research investigates the potential for energy recovery and the emission profiles of LSW combustibles via steam gasification at various temperatures (700, 750, 800, and 850 °C) and combustion at 850 °C, utilizing a fixed-bed reactor and TG-DSC analysis. Our findings indicate that steam gasification conducted at 850 °C yields a high-quality syngas with a hydrogen concentration of 46.
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