Interfaces between complex oxides constitute a unique playground for two-dimensional electron systems (2DESs), where superconductivity and magnetism can arise from combinations of bulk insulators. The 2DES at the LaAlO/SrTiO interface is one of the most studied in this regard, and its origin is determined by the polar field in LaAlO as well as by the presence of point defects, like oxygen vacancies and intermixed cations. These defects usually reside in the conduction channel and are responsible for a decrease of the electronic mobility. In this work, we use an amorphous WO overlayer to obtain a high-mobility 2DES in WO/LaAlO/SrTiO heterostructures. The studied system shows a sharp insulator-to-metal transition as a function of both LaAlO and WO layer thickness. Low-temperature magnetotransport reveals a strong magnetoresistance reaching 900% at 10 T and 1.5 K, the presence of multiple conduction channels with carrier mobility up to 80 000 cm V s, and quantum oscillations of conductance.
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http://dx.doi.org/10.1021/acsami.7b13202 | DOI Listing |
Nat Commun
January 2025
Anhui Key Laboratory of Low-Energy Quantum Materials and Devices, High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences, Hefei, Anhui, China.
Nat Commun
January 2025
State Key Laboratory of Superlattices and Microstructures, Institute of Semiconductors, Chinese Academy of Sciences, Beijing, China.
The insulator-to-metal transition in VO has garnered extensive attention for its potential applications in ultrafast switches, neuronal network architectures, and storage technologies. However, the photoinduced insulator-to-metal transition remains controversial, especially whether a complete structural transformation from the monoclinic to rutile phase is necessary. Here we employ the real-time time-dependent density functional theory to track the dynamic evolution of atomic and electronic structures in photoexcited VO, revealing the emergence of a long-lived monoclinic metal phase under low electronic excitation.
View Article and Find Full Text PDFSci Rep
December 2024
International Center for Synchrotron Radiation Innovation Smart (SRIS), Tohoku University, Miyagi, 980-8572, Japan.
With the growing awareness of energy savings and consumption for a sustainable ecosystem, the concept of iontronics, that is, controlling electronic devices with ions, has become critically important. Composite devices made of ions and solid materials have been investigated for diverse applications, ranging from energy storage to power generation, memory, biomimetics, and neuromorphic devices. In these studies, three terminal transistor configurations with liquid electrolytes have often been utilized because of their simple device structures and relatively easy fabrication processes.
View Article and Find Full Text PDFNanophotonics
March 2024
Department of Materials Science and Engineering, City University of Hong Kong, Kowloon, Hong Kong, China.
ACS Appl Mater Interfaces
December 2024
Center for Hybrid Nanostructures, Universität Hamburg, Luruper Chaussee 149, 22607 Hamburg, Germany.
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