The combination of electron-rich diaminoalkynes and ditopic Lewis acids diboranes(4) leads to unusual uncatalysed diboration reactions involving internal Lewis adduct, zwitterion, and C-C bond formation. The products are novel multicyclic, charge-separated compounds with intramolecular dative bonds.
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Alkylideneborate zwitterions and C-C coupling by atypical diboration of electron-rich alkynes.
Chem Commun (Camb)
November 2017
Institute for Inorganic Chemistry, Julius-Maximilians-Universität Würzburg, Am Hubland, 97074 Würzburg, Germany.
The combination of electron-rich diaminoalkynes and ditopic Lewis acids diboranes(4) leads to unusual uncatalysed diboration reactions involving internal Lewis adduct, zwitterion, and C-C bond formation. The products are novel multicyclic, charge-separated compounds with intramolecular dative bonds.
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