Less is known about controls of sedimentary structures in groundwater As distributions in sedimentary aquifers, and quantitative description of relationship between sedimentary environment and high As groundwater (according to WHO, As>10μg/L) is a challenging issue. Three hundred and eighty-two hydrogeological borehole loggings (well depths of 50-300m) were collected and four hundred and ninety nine groundwater samples were taken to investigate controls of paleochannels on groundwater arsenic distribution in shallow aquifers of alluvial plain in the Hetao Basin. Results showed that the swing zone, formed by bursting, diversion and swing of ancient Yellow River course since the Late Pleistocene, has an obviously corresponding relationship with spatial variability of groundwater As in the Hetao Basin. "Swing Intensity Index" (S), which is firstly defined as the sum of clay-sand ratio (R) and the number of clay layers (N), can be used as the sedimentary facies symbol to establish the new recognition method for hosting high As groundwater. There is a positive correlation between the swing intensity index (S) of paleochannels and groundwater As concentrations. The swing zones of paleochannels with high S values represent hydrogeochemical characteristics of the strong reducing environment, serious evaporation, strong cation exchange, and the low infiltration recharge of surface water, which lead to enrichment of groundwater As in the shallow aquifers.
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http://dx.doi.org/10.1016/j.scitotenv.2017.09.182 | DOI Listing |
Water Res
January 2025
Key Laboratory of Groundwater Quality and Health (China University of Geosciences), Ministry of Education, Wuhan 430078, China; State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution, School of Environmental Studies, Wuhan 430078, China.
The contamination of groundwater with geogenic ammonium (NH) across various geological backgrounds has garnered significant attention, particularly in coastal aquifer systems. However, there remains a gap in our understanding of the mechanisms governing the spatial variability of NH in coastal groundwater at a macroscopic scale. In this study, we collected the sediment samples from two boreholes corresponding to high-NH-N and low-NH-N groundwater.
View Article and Find Full Text PDFGround Water
November 2024
Department of Geoscience, Aarhus University, 1672 Høegh-Guldbergs Gade 2, 8000, Aarhus, Denmark.
Small island communities often rely on groundwater as their primary source of fresh water. However, the limited land area and high proportion of coastal zones pose unique challenges to groundwater management. A detailed understanding of the subsurface structure can provide valuable insights into aquifer structure, groundwater vulnerability, saltwater intrusion, and the location of water resources.
View Article and Find Full Text PDFSci Total Environ
December 2024
School of Environmental Studies, China University of Geosciences, Wuhan 430078, China; State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution, Ministry of Ecology and Environment, Wuhan 430078, China.
High iodine groundwater occurs widely in the lower reaches of Yellow River floodplain, which has aroused public concern. The biogeochemical behavior of dissolved organic matter (DOM) plays a crucial role in the mobilizing iodine from aquifer media. In this study, the molecular composition of DOM in groundwater characterized by FT-ICR-MS, and the optical properties of organic matter obtained by combining three-dimensional fluorescence spectroscopy and parallel factor analysis (EEM ⁃ PARAFAC), were used to elucidate the effect of DOM on the migration and enrichment of iodine in groundwater in the eastern Henan Plain, which is located in the lower reaches of Yellow River floodplain, Northern China.
View Article and Find Full Text PDFEnviron Sci Technol
April 2023
State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution, Hubei Key Laboratory of Yangtze Catchment Environmental Aquatic Science, China University of Geosciences, Wuhan 430078, China.
Naturally occurring (i.e., geogenic) ammonium in groundwater has been widely detected globally, but the major controls on its regional distribution have been poorly characterized.
View Article and Find Full Text PDFSci Total Environ
September 2022
School of Water Conservancy and Environment, University of Jinan, 250022, China.
Abnormal levels of co-occurring arsenic (As), fluoride (F) and iodine (I) in groundwater at the Hetao Basin are geochemically unique. The abnormal distribution of As, F and I is obviously related to the sedimentary environment. It is necessary to study the enrichment mechanisms for the co-occurrence of As, F and I in groundwater under the influence of the sedimentary environment in Hetao Basin.
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