Aerosols affect the insolation at ground and thus the Aerosol Optical Depth (AOD, a measure of aerosol pollution) plays an important role on the variation of the Physiological Equivalent Temperature (PET) at locations with different aerosol climatology. The aerosol effects upon PET were studied for the first time at four East Asian cities by coupling a radiative transfer model and a human thermal comfort model which were previously well evaluated. Evident with the MODIS and AERONET AOD observations, the aerosol pollution at Beijing and Seoul was higher than at Chiayi (Taiwan) and Hong Kong. Based on the AERONET data, with background AOD levels the selected temperate cities had similar clear-sky PET values especially during summertime, due to their locations at similar latitudes. This also applied to the sub-tropical cities. Increase in the AOD level to the seasonal average one led to an increase in diffuse solar radiation and in turn an increase in PET for people living in all the cities. However, the heavy aerosol loading environment in Beijing and Seoul in summertime (AODs > 3.0 in episodic situations) reduced the total radiative flux and thus PET values in the cities. On the contrary, relatively lower episodic AOD levels in Chiayi and Hong Kong led to strong diffuse and still strong direct radiative fluxes and resulted in higher PET values, relative to those with seasonal averaged AOD levels. People tended to feel from "hot" to "very hot" during summertime when the AOD reached their average levels from the background level. This implies that in future aerosol effects add further burden to the thermal environment apart from the effects of greenhouse gas-induced global warming. Understanding the interaction between ambient aerosols and outdoor thermal environment is an important first step for effective mitigation measures such as urban greening to reduce the risk of human heat stress. It is also critical to make cities more attractive and enhancing to human well-being to achieve enhancing sustainable urbanization as one of the principal goals for the Nature-based Solutions.
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http://dx.doi.org/10.1016/j.envres.2017.07.036 | DOI Listing |
Sci Total Environ
January 2025
School of Agriculture and Biology, Shanghai Jiao Tong University, 800 Dongchuan Rd., Shanghai 200240, China; Shanghai Yangtze River Delta Eco-Environmental Change and Management Observation and Research Station, Ministry of Science and Technology, Ministry of Education, 800 Dongchuan Rd., Shanghai 200240, China; Shanghai Urban Forest Ecosystem Research Station, National Forestry and Grassland Administration, 800 Dongchuan Rd., Shanghai 200240, China; Key Laboratory for Urban Agriculture, Ministry of Agriculture and Rural Affairs, 800 Dongchuan Rd., Shanghai 200240, China. Electronic address:
Biogenic volatile organic compounds (BVOCs) are emitted by urban vegetation and can interact with anthropogenic pollutants to generate secondary organic aerosols (SOA) that are atmospheric pollutants in urban environments. In urban forests, SOA comprise up to 90 % of all fine aerosols (particulate matter smaller than 1 μm [PM]) in the summer. PM can greatly affect urban air quality and public health.
View Article and Find Full Text PDFChem Res Toxicol
January 2025
Department of Environmental Sciences, University of California, Riverside, California 92521, United States.
E-cigarette emissions, which contain a variety of hazardous compounds, contribute significantly to indoor air pollution and raise concerns about secondhand exposure to vaping byproducts. Compared to fresh vape emissions, our understanding of chemically aged products in indoor environments remains incomplete. Terpenes are commonly used as flavoring agents in e-liquids, which have the ability to react with the dominant indoor oxidant ozone (O) to produce reactive oxygenated byproducts and result in new particle formation.
View Article and Find Full Text PDFEnviron Pollut
January 2025
Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China, Qingdao, 266100, PR China; College of Chemistry and Chemical Engineering, Ocean University of China, Qingdao, 266100, PR China. Electronic address:
Antibiotic resistance genes (ARGs) have escalated to levels of concern worldwide as emerging environmental pollutants. Increasing evidence suggests that non-antibiotic antimicrobial substances expedite the spread of ARGs. However, the drivers and mechanisms involved in the generation and spread of ARGs in the atmosphere remain inadequately elucidated.
View Article and Find Full Text PDFEnviron Pollut
January 2025
College of Meteorology and Oceanography, National University of Defense Technology, Changsha, 410073, China.
Understanding the composition of mercury (Hg) in the atmosphere is important for confirming its sources and to preventing and reduce the production. To explore the morphological distribution characteristics of wet Hg concentrations in Xi'an Shaanxi Province, China, total Hg (THg), dissolved Hg (DTHg), reactive Hg (RTHg) and particulate-bound Hg (PTHg) (Hg insoluble in water) were measured at 72 precipitation in Xi'an from September 2020 to July 2022, and their average concentrations were 3.035 ± 3.
View Article and Find Full Text PDFJ Am Chem Soc
January 2025
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, IRDR International Center of Excellence on Risk Interconnectivity and Governance on Weather, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, Peoples' Republic of China.
Hydroxyl radical (·OH) plays a crucial role in atmospheric chemistry, regulating the oxidative potential and aerosol composition. This study reveals an unprecedented source of ·OH in the atmosphere: mineral dust-bearing microdroplet aerosols. We demonstrate that Kaolin clay particles in microdroplet aerosols trigger rapid ·OH production upon solar irradiation, with rates reaching an order of at least 10 M s.
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