We report the results of resonant magnetic XUV reflectivity experiments performed at the XUV free-electron laser FERMI. Circularly polarized XUV light with the photon energy tuned to the Fe M edge is used to measure resonant magnetic reflectivities and the corresponding -resolved asymmetry of a Permalloy/Ta/Permalloy trilayer film. The asymmetry exhibits ultrafast changes on 240 fs time scales upon pumping with ultrashort IR laser pulses. Depending on the value of the wavevector transfer , we observe both decreasing and increasing values of the asymmetry parameter, which is attributed to ultrafast changes in the vertical spin and charge density profiles of the trilayer film.
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http://dx.doi.org/10.1063/1.4990650 | DOI Listing |
Chem Sci
January 2025
School of Physical Science and Technology, ShanghaiTech University Shanghai 201210 China
The process of proton translocation in , triggered by light, is powered by the photoisomerization of all--retinal in bacteriorhodopsin (bR). The primary events in bR involving rapid structural changes upon light absorption occur within subpicoseconds to picoseconds. While the three-state model has received extensive support in describing the primary events between the H and K states, precise characterization of each excited state in the three-state model during photoisomerization remains elusive.
View Article and Find Full Text PDFNat Commun
January 2025
DST Unit of Nanoscience (DST UNS) and Thematic Unit of Excellence (TUE), Department of Chemistry, Indian Institute of Technology, Madras, Chennai, 600036, India.
We report the synthesis of [Ag(o-CBT)] abbreviated as Ag, a stable 8e⁻ anionic cluster with a unique Ag@Ag@Ag core-shell structure, where o-CBT is ortho-carborane-1-thiol. By substituting Ag atoms with Au and/or Cu at specific sites we created isostructural clusters [AuAg(o-CBT)] (AuAg), [AgCu(o-CBT)] (AgCu) and [AuAgCu(o-CBT)] (AuAgCu). These substitutions make systematic modulation of their structural and electronic properties.
View Article and Find Full Text PDFNature
January 2025
Department of Physics, Korea Advanced Institute of Science and Technology (KAIST), Daejeon, Korea.
A particle current generated by pumping in the absence of gradients in potential energy, density or temperature is associated with non-trivial dynamics. A representative example is charge pumping that is associated with the quantum Hall effect and the quantum anomalous Hall effect. Spin pumping, the spin equivalent of charge pumping, refers to the emission of a spin current by magnetization dynamics.
View Article and Find Full Text PDFThe interaction between ultrafast, tightly focused lasers and materials has garnered significant interest owing to its distinctive properties. In this study, we present a versatile methodology for the fabrication of tunable plasmonic nanostructures by employing a disordered gold nanoisland-dielectric-metal configuration, achieved through femtosecond laser printing. By reshaping the gold nanoislands and reconfiguring them into nanograting-like structures, the orientation of these nanostructures is influenced by the polarization of the femtosecond laser light, leading to controllable plasmon resonance and polarization-sensitive color display.
View Article and Find Full Text PDFEpsilon-near-zero (ENZ) materials, i.e., materials with a vanishing real part of the permittivity, have become an increasingly desirable platform for exploring linear and nonlinear optical phenomena in nanophotonic and on-chip environments.
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