Multivalued logic (MVL) devices/circuits have received considerable attention because the binary logic used in current Si complementary metal-oxide-semiconductor (CMOS) technology cannot handle the predicted information throughputs and energy demands of the future. To realize MVL, the conventional transistor platform needs to be redesigned to have two or more distinctive threshold voltages (Vs). Here, we report a finding: the photoinduced drain current in graphene/WSe heterojunction transistors unusually decreases with increasing gate voltage under illumination, which we refer to as the light-induced negative differential transconductance (L-NDT) phenomenon. We also prove that such L-NDT phenomenon in specific bias ranges originates from a variable potential barrier at a graphene/WSe junction due to a gate-controllable graphene electrode. This finding allows us to conceive graphene/WSe-based MVL logic circuits by using the I-V characteristics with two distinctive Vs. Based on this finding, we further demonstrate a light-triggered ternary inverter circuit with three stable logical states (ΔV of each state <0.05 V). Our study offers the pathway to substantialize MVL systems.
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http://dx.doi.org/10.1021/acsnano.7b02635 | DOI Listing |
J Am Chem Soc
December 2024
Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, College of Chemistry and Materials, iChem (Collaborative Innovation Center of Chemistry for Energy Materials), Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, 200433 Shanghai, China.
Strongly coupled interfaces in the epitaxial growth heteronanocrystals (HNCs) provide advanced functionalities regarding interface connection, electron transfer, and carrier separation. However, the majority of current nanocomposites primarily focus on a single heterojunction involving only two subunits, which hinders the achievement of optimized synergy energy transfer among more than two components. Herein, ternary NaGdF:Yb,Tm-TiO:F-FeO HNCs with dual-heterojunction were synthesized based on the crystal plane epitaxial growth strategy for boosting near-infrared (NIR)-triggered photo-chemodynamic therapy (PCDT).
View Article and Find Full Text PDFNano Lett
July 2024
Shandong Technology Center of Nanodevices and Integration, School of Integrated Circuit, Shandong University, Jinan 250101, China.
Chemistry
April 2023
NMPA Key Laboratory for Research and Evaluation of Innovative Drug, Henan Key Laboratory of Organic Functional Molecule and Drug Innovation, Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang, Henan, 453007, P. R. China.
Photonic disinfection, particularly near-infrared (NIR) light triggered antibacterial, has emerged as a highly promising solution for combating pathogenic microbes due to its spatiotemporal operability, safety, and low cost of apparatus. However, it remains challenging to construct NIR-responsive antibacterial agents with high light-converting efficacy and elucidate synergistic mechanisms. In this work, ultrathin two-dimensional (2D) BiOCl-Bi S -Cu S ternary heterostructures that can efficiently kill drug-resistant bacteria were synthesized by doping 0D Bi S and Cu S nanoparticles in the 2D BiOCl nanosheets via a facile one-pot hydrothermal method.
View Article and Find Full Text PDFActa Biomater
March 2022
Ministry of Education (MOE) Key Laboratory of Macromolecular Synthesis and Functionalization Department of Polymer Science and Engineering, Zhejiang University, Hangzhou 310027, China. Electronic address:
L-arginine (L-Arg) is an important nitric oxide (NO) donor, and its exploration in NO gas therapy has received widespread attention. Application of nano-platforms that can efficiently deliver L-Arg and induce its rapid conversion to NO becomes a predominant strategy to achieve promising therapeutic effects in tumor treatment. Herein, an enhanced nano-vesicular system of ternary synergistic treatment combining NO therapy, photodynamic therapy (PDT) along with mild photothermal therapy (MPTT) was developed for cancer therapy.
View Article and Find Full Text PDFBiosens Bioelectron
October 2020
School of Electrical and Information Engineering, Jiangsu University, Zhenjiang, 212013, China.
Developing new self-powered sensors is highly demanded for smart portable electronic devices. Herein, a novel visible-light-driven self-powdered aptasensor with a metal-ligand charge transfer (MLCT)-induced signal-off strategy was established for microcystin-LR (MC-LR) sensing. The aptasensor was based on a self-breathing-like dual photoelectrode photocatalytic fuel cell (PFC) that was assembled with visible-light responsive ternary NG-TiO-Ag and NG-BiOBr nanocomposites as photoelectrodes.
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