We report the successful demonstration of a hybrid system that combines pulsed laser deposition (PLD) and magnetron sputtering (MS) to deposit high quality thin films. The PLD and MS simultaneously use the same target, leading to an enhanced deposition rate. The performance of this technique is demonstrated through the deposition of titanium dioxide and bismuth-based perovskite oxide BiFeCrO (BFCO) thin films on Si(100) and LaAlO (LAO) (100). These specific oxides were chosen due to their functionalities, such as multiferroic and photovoltaic properties (BFCO) and photocatalysis (TiO). We compare films deposited by conventional PLD, MS and PLD combined with MS, and show that under all conditions the latter technique offers an increased deposition rate (+50%) and produces films denser (+20%) than those produced by MS or PLD alone, and without the large clusters found in the PLD-deposited films. Under optimized conditions, the hybrid technique produces films that are two times smoother than either technique alone.
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http://dx.doi.org/10.1038/s41598-017-02284-0 | DOI Listing |
Background: Malaria is the disease caused by intracellular parasites known as species and is mainly transmitted by blood sucking female mosquitoes. During pregnancy, malaria results in severe complications to the mother, the fetus and the newborn. Symptoms of malaria, such as fever, malaise, headache, nausea and vomiting, in pregnant women can be mistakenly attributed solely to pregnancy.
View Article and Find Full Text PDFThe optical permittivity of monocrystalline direct bandgap semiconductors can be described well by critical point models based on parabolic band approximation (CPPB). However, the optical permittivity of polycrystalline direct bandgap semiconductors like halide perovskite thin films requires a more precise description. Till now, only thermal bandgap fluctuation or exponential decay of density of states is incorporated into the CPPB model.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
Department of Chemical Engineering and Conn Center for Renewable Energy ResearchUniversity of Louisville, 132 Eastern Parkway, Louisville, Kentucky 40292, United States.
We report a silicon anode for lithium-ion batteries consisting of a layer of 100% nanotubes directly bonded to copper foil. The process involved silicon deposition on a sacrificial zinc oxide nanorod film and removal of zinc oxide to produce a nanotube film directly on thin copper foils. The thickness of resulting films ranged from 9 to 20 μm with Si nanotubes having diameters of 200-400 nm and lengths of 2-10 μm.
View Article and Find Full Text PDFSmall Methods
January 2025
Liquid Sunlight Alliance, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, Berkeley, CA, 94720, United States.
Copper-tantalate, CuTaO (CTO), shows significant promise as an efficient photocathode for multi-carbon compounds (C) production through photoelectrochemical (PEC) CO reduction, owing to its suitable energy bands and catalytic surface. However, synthesizing CTO poses a significant challenge due to its metastable nature and thermal instability. In this study, this challenge is addressed by employing a flux-mediated synthesis technique using a sodium-based flux to create sodium-doped CTO (Na-CTO) thin films, providing enhanced nucleation and stabilization for the CTO phase.
View Article and Find Full Text PDFNat Nanotechnol
January 2025
Key Laboratory of Bio-inspired Materials and Interfacial Science, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing, China.
The miniaturization of light-emitting diodes (LEDs) is pivotal in ultrahigh-resolution displays. Metal-halide perovskites promise efficient light emission, long-range carrier transport and scalable manufacturing for bright microscale LED (micro-LED) displays. However, thin-film perovskites with inhomogeneous spatial distribution of light emission and unstable surface under lithography are incompatible with the micro-LED devices.
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