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Efficient Electrocatalytic Reduction of CO by Nitrogen-Doped Nanoporous Carbon/Carbon Nanotube Membranes: A Step Towards the Electrochemical CO Refinery. | LitMetric
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Efficient Electrocatalytic Reduction of CO by Nitrogen-Doped Nanoporous Carbon/Carbon Nanotube Membranes: A Step Towards the Electrochemical CO Refinery.

Hong Wang Jia Jia Pengfei Song Qiang Wang Debao Li Shixiong Min Chenxi Qian Lu Wang Young Feng Li Chun Ma Tom Wu Jiayin Yuan Markus Antonietti Geoffrey A Ozin

Angew Chem Int Ed Engl

Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Centre for Inorganic and Polymeric Nanomaterials, Departments of Chemistry, Chemical Engineering and Applied Chemistry, and Electrical and Computing Engineering, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S3H6, Canada.

Published: June 2017

Herein we introduce a straightforward, low cost, scalable, and technologically relevant method to manufacture an all-carbon, electroactive, nitrogen-doped nanoporous-carbon/carbon-nanotube composite membrane, dubbed "HNCM/CNT". The membrane is demonstrated to function as a binder-free, high-performance gas diffusion electrode for the electrocatalytic reduction of CO to formate. The Faradaic efficiency (FE) for the production of formate is 81 %. Furthermore, the robust structural and electrochemical properties of the membrane endow it with excellent long-term stability.

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http://dx.doi.org/10.1002/anie.201703720DOI Listing

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