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Failure Modes of Flexible LiCoO Cathodes Incorporating Polyvinylidene Fluoride Binders with Different Molecular Weights.

ACS Appl Mater Interfaces

February 2024

School of Electrical, Computer and Energy Engineering, Arizona State University, Tempe, Arizona 85287, United States.

Understanding the mechanical failure modes of lithium-ion battery [Li-ion batteries (LIBs)] electrodes is exceptionally important for enabling high specific energy and flexible LIB technologies. In this work, the failure modes of lithium cobalt oxide (LCO) cathodes under repeated bending and the role of the polymer binder in improving the mechanical durability of the LCO electrodes for use in flexible LIBs are investigated. Mechanical and electrochemical evaluations of LCO electrodes (areal capacity of ≥2.

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