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Cyclometalated Au(III) complexes with alkynylphosphine oxide ligands: synthesis and photophysical properties.
Dalton Trans
January 2025
Institute of Chemistry, St Petersburg University, Universitetskii pr. 26, 198504 St. Petersburg, Russia.
A series of cyclometalated Au(III) complexes [Au(C^N^C)(C-L-P(O)Ph)] with C^N^C = 2,6-diphenylpyridine and alkynylphosphine oxide ligands (L = no linker, Au1; phenyl, Au2; biphenyl, Au3; naphthyl, Au4; anthracenyl, Au5) were synthesized and fully characterized by spectroscopic methods and single crystal XRD analysis. The complexes obtained exhibit triplet (Au1-Au3) and dual (Au4, Au5) emissions in solution, in the solid phase and in the PMMA film, whose characteristics depend on the linker's nature of the alkynylphosphine oxide ligand. The description of electronic transitions responsible for energy absorption and emission in Au(III) complexes was made on the basis of a detailed analysis of the results of DFT calculations and has shown to involve ILCT, LLCT and MLCT transitions of singlet and triplet nature.
View Article and Find Full Text PDFEvaporation Dynamics of Deionized Water Droplets on Hydrophobic Leaves.
Langmuir
January 2025
Tianjin Key Laboratory of Refrigeration Technology, Tianjin University of Commerce, Tianjin 300134, China.
Self-cleaning applications based on bionic surface designs requires an in-depth understanding of unique and complex wetting and evaporation processes of sessile droplets on natural biosurfaces. To this end, hydrophobic bamboo and Kalanchoe blossfeldiana leaves are excellent candidates for self-cleaning applications, but various properties, such as the heat and mass transfer processes during evaporation, remain unknown. Here, the dynamics of contact angle, radius, and heat and mass transfer during evaporation of sessile droplets on bamboo and Kalanchoe blossfeldiana leaves with roughness in the range 2.
View Article and Find Full Text PDF2-Amidophenolate and 2-Iminosemiquinone Radical-Coordinated Vanadyl Complex as Catholyte for Non-Aqueous Redox-Flow Batteries.
Chem Asian J
January 2025
Indian Institute of Technology Guwahati, Department of Chemistry, Department of Chemistry, 781039, Guwahati, INDIA.
Fulfilment of energy demand by utilizing renewable energy sources that do not contribute to the production of greenhouse gases is a step forward in mitigating global warming. However, with the energy sources being intermittent in nature, renewable energy needs to be stored effectively on a grid scale. In this context, the development of redox-flow batteries has emerged as a promising technology where charging and discharging processes are accomplished by the redox shuttling of the electrolytes, namely anolytes and catholytes.
View Article and Find Full Text PDFPartial migration is a phenomenon where migratory and resident individuals of the same species co-exist within a population, and has been linked to both intrinsic (e.g., genetic) as well as environmental factors.
View Article and Find Full Text PDFDuodromic atrioventricular reentry tachycardia: a case report of a rare adenosine insensitive supraventricular tachycardia.
Eur Heart J Case Rep
January 2025
Arrhythmology, Pacing and Electrophysiology Unit, Cardiology Service, Santa Marta Hospital, Central Lisbon Hospital University Centre, R. de Santa Marta 50, Lisboa 1169-024, Portugal.
Background: Accessory pathways (AP) are associated with an increased risk of atrioventricular reentry tachycardia (AVRT), presenting as a wide QRS tachycardia if the mechanism is antidromic. Rarely, AVRT may not respond to adenosine, suggesting a duodromic mechanism if the patient has multiple APs. Herein, we present a case of a male patient with multiple APs, wide QRS complex tachycardia, and resistance to adenosine.
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