Studies of magnetization dynamics have incessantly facilitated the discovery of fundamentally novel physical phenomena, making steady headway in the development of magnetic and spintronics devices. The dynamics can be induced and detected electrically, offering new functionalities in advanced electronics at the nanoscale. However, its scattering mechanism is still disputed. Understanding the mechanism in thin films is especially important, because most spintronics devices are made from stacks of multilayers with nanometer thickness. The stacks are known to possess interfacial magnetic anisotropy, a central property for applications, whose influence on the dynamics remains unknown. Here, we investigate the impact of interfacial anisotropy by adopting CoFeB/MgO as a model system. Through systematic and complementary measurements of ferromagnetic resonance (FMR) on a series of thin films, we identify narrower FMR linewidths at higher temperatures. We explicitly rule out the temperature dependence of intrinsic damping as a possible cause, and it is also not expected from existing extrinsic scattering mechanisms for ferromagnets. We ascribe this observation to motional narrowing, an old concept so far neglected in the analyses of FMR spectra. The effect is confirmed to originate from interfacial anisotropy, impacting the practical technology of spin-based nanodevices up to room temperature.
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http://dx.doi.org/10.1073/pnas.1613864114 | DOI Listing |
Chem Commun (Camb)
March 2025
Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln, Lincoln, NE, 68588-0299, USA.
Capitalizing on the nonvolatile, nanoscale controllable polarization, ferroelectric perovskite oxides can be integrated with various functional materials for designing emergent phenomena enabled by charge, lattice, and polar symmetry mediated interfacial coupling, as well as for constructing novel energy-efficient electronics and nanophotonics with programmable functionalities. When prepared in thin film or membrane forms, the ferroelectric instability of these materials is highly susceptible to the interfacial electrostatic and mechanical boundary conditions, resulting in tunable polarization fields and Curie temperatures and domain formation. This review focuses on two types of ferroelectric oxide-based heterostructures: the epitaxial perovskite oxide heterostructures and the ferroelectric oxides interfaced with two-dimensional van der Waals materials.
View Article and Find Full Text PDFSmall
March 2025
School of Chemistry and Chemical Engineering, Southwest Petroleum University, 8 Xindu Avenue, Xindu District, Chengdu, Sichuan, 610500, P. R. China.
Janus hollow microstructures have been widely used in chemistry, medicine, biology, and materials science because of their anisotropy and hollow structure. Constructing multiple types of hollow microstructures and establishing structure-property relationships remain challenging. Here, the present authors develop a one-pot polymerization strategy for constructing Janus hollow microstructures in which deep eutectic solvents (DESs) completely replace water as the continuous phase.
View Article and Find Full Text PDFACS Nano
March 2025
Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Academy for Engineering & Technology, Advanced Coatings Research Center of Ministry of Education of China, Fudan University, Shanghai 200438, China.
Sharp corners and edges with high surface curvature provide low-dimensional nanosized materials with special static magnetic properties. However, the surface engineering of their high-frequency magnetic response remains challenging, and the underlying mechanism requires further clarification. In this study, we propose a template-aided surface reorganization strategy for integrating surfaces with different curvatures into one permalloy architecture.
View Article and Find Full Text PDFNat Commun
February 2025
Department of Physics, Columbia University, New York, NY, USA.
Graphene is a privileged 2D platform for hosting confined light-matter excitations known as surface plasmon polaritons (SPPs), as it possesses low intrinsic losses and a high degree of optical confinement. However, the isotropic nature of graphene limits its ability to guide and focus SPPs, making it less suitable than anisotropic elliptical and hyperbolic materials for polaritonic lensing and canalization. Here, we present graphene/CrSBr as an engineered 2D interface that hosts highly anisotropic SPP propagation across mid-infrared and terahertz energies.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
February 2025
School of Materials Science and Engineering, Zhejiang University, Hangzhou, 310027, China.
Metal anodes are of profound impact towards the realization of energy-dense rechargeable batteries. However, the "hostless" metal redox always presents the disordered plating/stripping, aggravated by the side reactions and local anisotropy that cause the formation of excessive dendrites/voids and quickly lead to battery failure. Here we report step-edge guided homoepitaxy enabling ordered layer-by-layer Zn plating/stripping regardless of the (dis)charging conditions.
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