Hybrid perovskite CHNHPbI has attracted extensive research interests in optoelectronic devices in recent years. Herein an inkjet printing method has been employed to deposit a perovskite CHNHPbI layer. By choosing the proper solvent and controlling the crystal growth rate, hybrid perovskite CHNHPbI nanowires, microwires, a network, and islands were synthesized by means of inkjet printing. Electrode-gap-electrode lateral-structured photodetectors were fabricated with these different crystals, of which a hybrid perovskite microwire-based photodetector would balance the uniformity and low defects to obtain a switching ratio of 16000%, responsivity of 1.2 A/W, and normalized detectivity of 2.39 × 10 Jones at a light power density of 0.1 mW/cm. Furthermore, the hybrid perovskite microwire-based photodetector arrays were fabricated and applied in an imaging sensor, from which the clear mapping of the light source signal was successfully obtained. This work paves the way for the realization of low-cost, solution-processed, and high-performance hybrid perovskite-based photodetector arrays.

Download full-text PDF

Source
http://dx.doi.org/10.1021/acsami.7b01379DOI Listing

Publication Analysis

Top Keywords

hybrid perovskite
20
perovskite chnhpbi
16
photodetector arrays
12
inkjet printing
8
perovskite microwire-based
8
microwire-based photodetector
8
hybrid
6
perovskite
6
inkjet-printed photodetector
4
arrays based
4

Similar Publications

Hybridization effects on the magnetic ground state of ruthenium in double perovskite LaZnRuTiO.

J Phys Condens Matter

January 2025

School of Materials Science, Indian Association for the Cultivation of Science, Calcutta 700 032, Kolkata, West Bengal, 700032, INDIA.

An exotic quantum mechanical ground state, i.e. the nonmagnetic= 0 state, has been predicted for higher transition metal tsystems, due to the influence of strong spin-orbit coupling (SOC) or in other words, due to unquenched orbital moment contribution.

View Article and Find Full Text PDF

Organic-inorganic formamidinium lead triiodide (FAPbI) hybrid perovskite quantum dots (QDs) have garnered considerable attention in the photovoltaic field due to their narrow bandgap, exceptional environmental stability, and prolonged carrier lifetime. Unfortunately, their insulating ligands and surface vacancy defects pose significant obstacles to efficient charge transfer across device interfaces. In this work, an electrostatic harmonization strategy at the interface using a donor-acceptor dipole molecular attachment to achieve enhanced charge separation capabilities on the QD surface is ventured.

View Article and Find Full Text PDF

Dual-Phase Ligand Engineering Enables 18.21% FAPbI Quantum Dot Solar Cells.

Adv Mater

January 2025

Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory of Advanced Negative Carbon Technologies, Soochow University, 199 Ren-Ai Road, Suzhou Industrial Park, Suzhou, Jiangsu, 215123, P. R. China.

Formamidinium lead triiodide (FAPbI) perovskite quantum dot (PQD) are promising candidate for high-performing quantum dot photovoltaic due to its narrow bandgap, high ambient stability, and long carrier lifetime. However, the carrier transport blockage and nonradiative recombination loss, originating from the high-dielectric ligands and defects/trap states on the FAPbI PQD surface, significantly limit the efficiency and stability of its photovoltaic performance. In this work, through exploring dual-site molecular ligands, namely 2-thiophenemethylammonium iodide (2-TM) and 2-thiopheneethylammonium iodide (2-TE), a dual-phase synergistic ligand exchange (DSLE) protocol consisting of both solution-phase and solid-state ligand engineering is demonstrated.

View Article and Find Full Text PDF

Heavy metal pollution is a major environmental and health problem due to the toxicity and persistence of metals such as lead, mercury, cadmium, and arsenic in water, soil, and air. Advances in sensor technology have significantly improved the detection and quantification of heavy metals, providing real-time monitoring and mitigation tools. This review explores recent developments in heavy metal detection, focusing on innovative uses of immobilized chromogenic reagents, nanomaterials, perovskites, and nanozymes.

View Article and Find Full Text PDF

Rare Earth Complex-Based Functional Materials: From Molecular Design and Performance Regulation to Unique Applications.

Acc Chem Res

January 2025

State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Nonferrous Metal Chemistry and Resources Utilization of Gansu Province, College of Chemistry and Chemical Engineering, Lanzhou University, Lanzhou 730000, China.

ConspectusRare earth (RE) elements, due to their unique electronic structures, exhibit excellent optical, electrical, and magnetic properties and thus have found widespread applications in the fields of electronics, optics, and biomedicine. A significant advancement in the use of RE elements is the formation of RE complexes. RE complexes, created by the coordination of RE ions with organic ligands, not only offer high molecular design flexibility but also incorporate features such as a broad absorption band and efficient energy transfer of organic ligands.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!