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Intensifying Interfacial Reverse Hydrogen Spillover for Boosted Electrocatalytic Nitrate Reduction to Ammonia.
Angew Chem Int Ed Engl
January 2025
Shandong university, School of Chemistry and Chemical Engineering, No 27, Shandananlu,, 250100, Jinan, CHINA.
Rational regulation of active hydrogen (*H) behavior is crucial for advancing electrocatalytic nitrate reduction reaction (NO3RR) to ammonia (NH3), yet in-depth understanding of the *H generation, transfer, and utilization remains ambiguous, and explorations for *H dynamic optimization are urgently needed. Herein we engineer a Ni3N nanosheet array intimately decorated with Cu nanoclusters (NF/Ni3N-Cu) for remarkably boosted NO3RR. From comprehensive experimental and theoretical investigations, the Ni3N moieties favors water dissociation to generate *H, and then *H can rapidly transfer to the Cu via unique reverse hydrogen spillover mediating interfacial Ni-N-Cu bridge bond, thus increasing *H coverage on the Cu site for subsequent deoxygenation/hydrogenation.
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Department of Clinical Nursing, The First Affiliated Hospital of China Medical University, Shenyang, Liaoning, China.
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View Article and Find Full Text PDFInfectious Risk in Pediatric Emergency Departments in Italy: A Survey by the Italian Society for Pediatric Emergency and Urgent Medicine (SIMEUP) on Available Preventive and Diagnostic Tools.
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Pediatric Clinic, Department of Medicine and Surgery, University of Parma, Via Gramsci, 14, 43125 Parma, Italy.
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