We present a theoretical investigation of terahertz (THz) generation in laser-induced gas plasmas. The work is strongly motivated by recent experimental results on microplasmas, but our general findings are not limited to such a configuration. The electrons and ions are created by tunnel ionization of neutral atoms, and the resulting plasma is heated by collisions. Electrons are driven by electromagnetic, convective, and diffusive sources and produce a macroscopic current which is responsible for THz emission. The model naturally includes both ionization current and transition-Cherenkov mechanisms for THz emission, which are usually investigated separately in the literature. The latter mechanism is shown to dominate for single-color multicycle laser pulses, where the observed THz radiation originates from longitudinal electron currents. However, we find that the often discussed oscillations at the plasma frequency do not contribute to the THz emission spectrum. In order to predict the scaling of the conversion efficiency with pulse energy and focusing conditions, we propose a simplified description that is in excellent agreement with rigorous particle-in-cell simulations.
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Sci Rep
January 2025
Departament de Fisica de la Materia Condensada, University of Barcelona, Marti i Franquès 1, 08028, Barcelona, Spain.
We present a nonlinear model of thermal field emission in resonant tunneling nanostructures with multiple barriers and potential wells, based on an accurate determination of the quantum potential shape and a rigorous solution of the Schrödinger equation, while considering thermal balance. The model applies to vacuum and semiconductor resonant tunnel diode and triode structures with two and three electrodes and to the general case of two-way tunneling with electrode heating. The complete balance of heat release and transfer is accounted for, with heat transport considered ballistic.
View Article and Find Full Text PDFTerahertz (THz) generation via photomixing on photoconductive antenna using twin delayed chirped pulses provides a long THz pulse with a narrow bandwidth. To generate a long pulse with a broad bandwidth, we propose a new, to the best of our knowledge, method that combines two long optical pulses with opposite chirps. The pulses exhibit temporal distributions of their instantaneous frequencies with opposite slopes.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
State Key Laboratory of Optoelectronic Materials and Technologies, School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, P. R. China.
Terahertz (THz) emission arising from the second-order nonlinear photocurrent effects in two-dimensional quantum materials has attracted significant attention due to its high efficiency and ease of polarization manipulation. However, in centrosymmetric quantum materials, the terahertz emission is typically suppressed, caused by the directional symmetry of the photocurrent generated under femtosecond laser excitation. In this work, we report that wafer-scale type-II Dirac semimetal PtTe with lattice centrosymmetry exhibits remarkably high THz emission efficiency (2 orders of magnitude greater than that of a ZnTe nonlinear crystal with equivalent thickness) and pronounced polarization sensitivity at room temperature.
View Article and Find Full Text PDFHolographically designed aperiodic lattices (ALs) have proven to be an exciting engineering technique for achieving electrically switchable single- or multi-frequency emissions in terahertz (THz) semiconductor lasers. Here, we employ the nonlinear transfer matrix modeling method to investigate multi-wavelength nonlinear (sum- or difference-) frequency generation within an integrated THz (idler) laser cavity that also supports optical (pump and signal) waves. The laser cavity includes an aperiodic lattice, which engineers the idler photon lifetimes and effective refractive indices.
View Article and Find Full Text PDFAdv Mater
December 2024
Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, China.
The orbital Hall effect originating from light materials with weak spin-orbit coupling, has attracted considerable interest in spintronic applications. Recent studies demonstrate that orbital currents can be generated from charge currents through the orbital Hall effect in ferromagnetic materials. However, the generation of orbital currents in antiferromagnets has so far been elusive.
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