We study Coulomb interacting electrons confined in polygonal quantum rings. We focus on the interplay of localization at the polygon corners and Coulomb repulsion. Remarkably, the Coulomb repulsion allows the formation of in-gap states, i.e., corner-localized states of electron pairs or clusters shifted to energies that were forbidden for non-interacting electrons, but below the energies of corner-side-localized states. We specify conditions allowing optical excitation to those states.
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http://dx.doi.org/10.1038/srep40197 | DOI Listing |
Angew Chem Int Ed Engl
December 2024
Department of Chemistry, Tsinghua University, 100084, Beijing, P. R. China.
A golden fullerene with a composition of [Au(PhP)(5-CF-Hpa)] (CFCOO) (5-CF-Hpa=5-trifluoropyridyl-2-amine) (Au) has been synthesized with pyridylamino and phosphine ligands as the protecting agents. Single crystal X-ray structural analysis reveals that the cluster has a D Au core, which can be depicted as a centered core-shell structure Au@Au@Au. The 41 Au atoms of the Au@Au core-shell can be derived from placing a gold atom in the center of each polygon of C (D).
View Article and Find Full Text PDFMicrosc Microanal
October 2024
Central Facility for Materials Science Electron Microscopy, Universität Ulm, Einsteinallee 11, 89081 Ulm, Germany.
In this study, we explore the dynamics of grain boundaries in nanocrystalline carbon monolayers, focusing on their variation with electron beam energy and electron dose rate in a spherical and chromatic aberration-corrected transmission electron microscope. We demonstrate that a clean surface, a high-dose rate, and a 60 keV electron beam are essential for precise local control over the dynamics of grain boundaries. The structure of these linear defects has been evaluated using neural network-generated polygon mapping.
View Article and Find Full Text PDFNanomaterials (Basel)
September 2024
State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, China.
In this paper, multifunctional, multilevel phase plates of quartz substrate were efficiently prepared by using a newly developed polygon scanner-based femtosecond laser photolithography system combined with inductively coupled discharge plasma reactive-ion etching (ICP-RIE) technology. The femtosecond laser photolithography system can achieve a scanning speed of 5 m/s and a preparation efficiency of 15 cm/h while ensuring an overlay alignment accuracy of less than 100 nm and a writing resolution of 500 nm. The ICP-RIE technology can control the etching depth error within ±5 nm and the mask-to-mask edge error is less than 1 μm.
View Article and Find Full Text PDFNanoscale Adv
September 2024
Plasmonics and Perovskites Laboratory, Indian Institute of Technology Kanpur UP 208016 India +91-512-259-6599.
Optical vortices have a topologically charged phase singularity and zero intensity distribution in the centre. Optical vortex creation is regarded as a significant means for information transmission for applications in quantum computing, encryption, optical communication, In this study, using finite-difference time-domain (FDTD) simulation, we calculated the electric field intensity and phase distribution of 2D lattices of optical vortices generated from various polygonal plasmonic lens structures using surface states of a Weyl semimetal (MoTe). It was shown that a hexagonal lens is the best performing plasmonic lens.
View Article and Find Full Text PDFEntropy (Basel)
February 2024
Center for Coherence and Quantum Optics, Department of Physics and Astronomy, University of Rochester, Rochester, NY 14627, USA.
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