Energy-storage technologies such as lithium-ion batteries and supercapacitors have become fundamental building blocks in modern society. Recently, the emerging direction toward the ever-growing market of flexible and wearable electronics has nourished progress in building multifunctional energy-storage systems that can be bent, folded, crumpled, and stretched while maintaining their electrochemical functions under deformation. Here, recent progress and well-developed strategies in research designed to accomplish flexible and stretchable lithium-ion batteries and supercapacitors are reviewed. The challenges of developing novel materials and configurations with tailored features, and in designing simple and large-scaled manufacturing methods that can be widely utilized are considered. Furthermore, the perspectives and opportunities for this emerging field of materials science and engineering are also discussed.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1002/adma.201603436 | DOI Listing |
Nat Commun
January 2025
Key Laboratory of Flexible Electronics (KLOFE) & Institute of Advanced Materials (IAM), Nanjing Tech University (NanjingTech), Nanjing, China.
Fully π-conjugated polymers consisting of plane and rigid aromatic units present a fantastic optoelectronic property, a promising candidate for printed and flexible optoelectronic devices. However, obtaining high-performance conjugated polymers with an excellent intrinsically flexible and printable capacity is a great challenge due to their inherent coffee-ring effect and brittle properties. Here, we report an asymmetric substitution strategy to improve the printable and stretchable properties of deep-blue light-emitting conjugated polymers with a strong inter-aggregate capillary interaction for flexible printed polymer light-emitting diodes.
View Article and Find Full Text PDFInt J Biol Macromol
December 2024
State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Applied Chemistry, Hebei Key Laboratory of Nanobiotechnology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse, Yanshan University, Qinhuangdao 066004, China. Electronic address:
Preparation of ion-conductive hydrogels with excellent mechanics, good conductivity and adhesiveness is promising for flexible sensors, but remains a challenge. Here, we prepare a self-adhesive and ion-conductive hydrogel by introducing cellulose nanofibers (CNF) and ZnSO into a covalently-crosslinked poly (acrylamide-co-2-acrylamide-2-methyl propane sulfonic acid) (P(AM-co-AMPS)) network. Owing to the hydrogen bonding and metal coordination interactions among P(AM-co-AMPS) chains, CNF, and Zn, the resulting P(AM-co-AMPS)/CNF/ZnSO hydrogel exhibits high stretchability (1092 %), high toughness (244 kJ m), and skin-like elasticity (3.
View Article and Find Full Text PDFInt J Biol Macromol
December 2024
College of Materials Science and Engineering, Nanjing Tech University, Nanjing 210009, China.
Conductive hydrogels have great potential for applications in flexible wearable sensors due to the combination of biocompatibility, mechanical flexibility and electrical conductivity. However, constructing conductive hydrogels with high toughness, low hysteresis and skin-like modulus simultaneously remains challenging. In the present study, we prepared a tough and conductive polyacrylamide/pullulan/ammonium sulfate hydrogel with a semi-interpenetrating network.
View Article and Find Full Text PDFSci Rep
December 2024
Department of Engineering, Norfolk State University, Norfolk, USA.
We report a controlled deposition process using atmospheric plasma to fabricate silver nanoparticle (AgNP) structures on polydimethylsiloxane (PDMS) substrates, essential for stretchable electronic circuits in wearable devices. This technique ensures precise printing of conductive structures using nanoparticles as precursors, while the relationship between crystallinity and plasma treatment is established through X-ray diffraction (XRD) analysis. The XRD studies provide insights into the effects of plasma parameters on the structural integrity and adhesion of AgNP patterns, enhancing our understanding of substrate stretchability and bendability.
View Article and Find Full Text PDFGels
November 2024
Electro-Medical Equipment Research Division, Korea Electrotechnology Research Institute (KERI), Ansan 15588, Republic of Korea.
Shape-memory materials are widely utilized in biomedical devices and tissue engineering, particularly for their ability to undergo predefined shape changes in response to external stimuli. In this study, a shape-transformable organohydrogel was developed by incorporating a gallium mesh into a polyacrylamide/alginate/glycerol matrix. The gallium mesh, which transitions between solid and liquid states at moderate temperatures (~29.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!