Use of ultra-low-background capabilities at Pacific Northwest National Laboratory provide enhanced sensitivity for measurement of low-activity sources of tritium and radiocarbon using proportional counters. Tritium levels are nearly back to pre-nuclear test backgrounds (~2-8 TU in rainwater), which can complicate their dual measurement with radiocarbon due to overlap in the beta decay spectra. We present results of single-isotope proportional counter measurements used to analyze a dual-isotope methane sample synthesized from ~120mg of HO and present sensitivity results.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1016/j.apradiso.2016.12.033 | DOI Listing |
Nat Commun
October 2024
Department of Technical Biogeochemistry, Helmholtz Centre for Environmental Research - UFZ, Leipzig, Germany.
J Environ Radioact
December 2024
"Horia Hulubei" National Institute for Physics and Nuclear Engineering, Life and Environmental Physics Department, 30 Reactorului St., Bucharest-Magurele, POB MG-6, RO-077125, Romania. Electronic address:
Any major nuclear facility must ensure the conservation of biodiversity regarding radiation protection of biota. A special concern is for tritium (H) and radiocarbon (C) transfer in wild mammals, birds and reptiles. Hydrogen and carbon are the main components of biological tissues and enter the life cycle.
View Article and Find Full Text PDFSci Total Environ
December 2024
IRSN, PSE-ENV/STAAR/LRTA, BP 159, CEA Cadarache, 13115 Saint-Paul-les-Durance, France.
Carbon-14 (C) has a natural origin but is also anthropogenically released from civil nuclear facilities. Due to its long decay period (half-life: 5700 ± 30 years), it is a persistent radionuclide in the environment. In rivers, the complex speciation of carbon makes the fate of industrial C difficult to track.
View Article and Find Full Text PDFSci Total Environ
July 2024
University of Ottawa, 75 Laurier Ave E, Ottawa, ON K1N 6N5, Canada.
Unconventional hydrocarbon production has sparked public concerns for several years, especially regarding potential potable groundwater contamination by hydrocarbons, brines, and various chemicals related to hydraulic fracturing operations. One possible contamination mechanism is upward migration of deep-seated contaminants over large vertical distances, through preferential pathways such as leaky well casings or permeable geological faults. In New Brunswick (Canada), thermogenic hydrocarbons and brackish water were previously reported in shallow water wells, some of them located close to unconventional gas wells or to major faults, but the exact origin of these fluids remained uncertain.
View Article and Find Full Text PDFSci Total Environ
April 2024
International Atomic Energy Agency, Department of Nuclear Sciences and Applications, Division of Physical and Chemical Sciences, Isotope Hydrology Section, Vienna International Centre, PO Box 100, 1400, Vienna, Austria.
Fundamental approaches to the study of groundwater rely on investigating the spatial and temporal distribution of stable and radioactive isotopes and other anthropogenic compounds in natural waterbodies. The most often used tracers for estimating groundwater flow paths and residence times, groundwater/surface water interaction as well as tracing chemical (contamination) sources include stable isotopes of water (δ O and δ H), radiocarbon (C; t = 5730 a), tritium (H; t = 12.43 a) as well as unreactive fluorine-containing gases (e.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!