The sub-cycle dynamics of electrons driven by strong laser fields is central to the emerging field of attosecond science. We demonstrate how the dynamics can be probed through high-order harmonic generation, where different trajectories leading to the same harmonic order are initiated at different times, thereby probing different field strengths. We find large differences between the trajectories with respect to both their sensitivity to driving field ellipticity and resonant enhancement. To accurately describe the ellipticity dependence of the long trajectory harmonics we must include a sub-cycle change of the initial velocity distribution of the electron and its excursion time. The resonant enhancement is observed only for the long trajectory contribution of a particular harmonic when a window resonance in argon, which is off-resonant in the field-free case, is shifted into resonance due to a large dynamic Stark shift.
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http://dx.doi.org/10.1038/srep39006 | DOI Listing |
Rev Sci Instrum
January 2025
Université Paris-Saclay, CNRS, Institut des Sciences Moléculaires d'Orsay, 91405 Orsay, France.
We present the design of a VMI spectrometer optimized for attosecond spectroscopy in the 0-40 eV energy range. It is based on a compact three-electrode configuration where the lens shape, size, and material have been optimized using numerical simulations to improve the spectral resolution by a factor of ∼5 relative to the initial design [Eppink and Parker, Rev. Sci.
View Article and Find Full Text PDFJ Phys Chem A
January 2025
School of Physics and Electronic Technology, Liaoning Normoal University, Dalian 116081, People's Republic of China.
Photolysis of energetic materials offers safer and more controllable advantages compared to traditional ignition methods. Tracking the group and electron dynamics during the photolysis of energetic materials is currently a hot and challenging topic. In this work, we used a time-dependent density functional theory (TDDFT) to study the high-order Harmonic generation (HHG) dynamics induced by strong laser interaction with an isolated CHNO molecule with varying C-N bond lengths.
View Article and Find Full Text PDFNat Commun
December 2024
Wuhan Institute of Physics and Mathematics, Innovation Academy for Precision Measurement Science and Technology, Chinese Academy of Sciences, Wuhan, 430071, China.
Electron diffraction spectroscopy is a fundamental tool for investigating quasicrystal structures, which unveils the quasiperiodic long-range order. Nevertheless, it falls short in effectively distinguishing separate local isomorphism classes. This is a long outstanding problem.
View Article and Find Full Text PDFBrain Struct Funct
December 2024
Sensory and Motor Systems Research Group, Korea Brain Research Institute, Daegu, South Korea.
Vocal learners, including humans and songbirds, acquire their complex vocalizations by accurately memorizing and imitating the vocal patterns of other individuals. In songbirds, the caudomedial nidopallium (NCM), considered the secondary auditory region, has been suggested to play a critical role in memorizing and recognizing the songs of tutors. However, the mechanisms by which NCM neurons encode the acoustic information of tutor song are not yet fully understood.
View Article and Find Full Text PDFNanophotonics
August 2024
Friedrich-Schiller University Jena, Jena, Germany.
High-order harmonic generation (HHG) in solids opens new frontiers in ultrafast spectroscopy of carrier and field dynamics in condensed matter, picometer resolution structural lattice characterization and designing compact platforms for attosecond pulse sources. Nanoscale structuring of solid surfaces provides a powerful tool for controlling the spatial characteristics and efficiency of the harmonic emission. Here we study HHG in a prototypical phase-change material GeSbTe (GST).
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